Post-Ionization Dynamics of the Polar Molecule OCS in Asymmetric Laser Fields Article Swipe

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Tomoyuki Endo , Karl Michael Ziems , Martin Richter , Friedrich Georg Fröbel , Akiyoshi Hishikawa , Stefanie Gräfe , François Légaré , Heide Ibrahim ·

YOU? · · 2022 · Open Access · · DOI: https://doi.org/10.3389/fchem.2022.859750

We have investigated the dissociation mechanisms of the prototypical heavy polar molecule OCS into the two break-up channels of the dication, OCS 2+ → O + + CS + and OC + + S + , in phase-locked two-color intense laser fields. The branching ratio of the breaking of the C–O and C–S bonds followed a pronounced 2 π -oscillation with a modulation depth of 11%, depending on the relative phase of the two-color laser fields. The fragment ejection direction of both break-up channels reflects the anisotropy of the tunneling ionization rate, following a 2 π -periodicity, as well. The two dissociation pathways in the C–S bond breaking channel show different phase dependencies of the fragment ejection direction, which are assigned to post-ionization dynamics. These observations, resulting from the excitation with asymmetric two-color intense laser fields, supported by state-of-the-art theoretical simulations, reveal the importance of post-ionization population dynamics in addition to tunneling ionization in the molecular fragmentation processes, even for heavy polar molecules.

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Ionization Molecule Polar Laser Chemical physics Dynamics (music) Chemistry Atomic physics Molecular physics Physics Materials science Optics Ion Organic chemistry Quantum mechanics Acoustics

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Type: article
Language: en
Landing Page: https://doi.org/10.3389/fchem.2022.859750
OA Status: gold
Cited By: 12
References: 71
Related Works: 10
OpenAlex ID: https://openalex.org/W4226068798

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DOI: https://doi.org/10.3389/fchem.2022.859750

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Title: Post-Ionization Dynamics of the Polar Molecule OCS in Asymmetric Laser Fields

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Language: en

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Publication year: 2022

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Publication date: 2022-04-08

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Authors: Tomoyuki Endo, Karl Michael Ziems, Martin Richter, Friedrich Georg Fröbel, Akiyoshi Hishikawa, Stefanie Gräfe, François Légaré, Heide Ibrahim

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Landing page: https://doi.org/10.3389/fchem.2022.859750

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Concepts: Ionization, Molecule, Polar, Laser, Chemical physics, Dynamics (music), Chemistry, Atomic physics, Molecular physics, Physics, Materials science, Optics, Ion, Organic chemistry, Quantum mechanics, Acoustics

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Cited by: 12

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