Precisely visit the performance modulation of functionalized separator in Li-S batteries via consecutive multiscale analysis Article Swipe
Zhangxiang Hao
,
Jie Chen
,
Xuekun Lu
,
Liqun Kang
,
Chun Tan
,
Ruoyu Xu
,
Lixia Yuan
,
Dan J. L. Brett
,
Paul R. Shearing
,
Feng Ryan Wang
,
Yunhui Huang
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.ensm.2022.04.003
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.ensm.2022.04.003
Despite progress of functionalized separator in preventing the shuttle effect and promoting the sulfur utilization, the precise and non-destructive investigation of structure-function-performance associativity remains limited so far in Li-S batteries. Here, we build consecutive multiscale analysis via combining X-ray absorption fine structure (XAFS) and X-ray computational tomography (CT) techniques to precisely visit the structure-function-performance relationship. XAFS measurement offers the atomic scale changes in the chemical structure and environment. Moreover, a non-destructive technique of X-ray CT proves the functionalized separator role for microscopic scale, which is powerful chaining to bridge the chemical structures of the materials with the overall performance modulation of cells. Benefiting from this consecutive multiscale analysis, we report that the uniform doping of Sr2+ into the perovskite LaMnO3-δ material changes the Mn oxidation states and conductivity (chemical structure), leading to effective lithium polysulfide trapping and accelerated sulfur redox (separator function), and resulting in outstanding cell performance.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.ensm.2022.04.003
- OA Status
- hybrid
- Cited By
- 15
- References
- 42
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4223994878
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4223994878Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.ensm.2022.04.003Digital Object Identifier
- Title
-
Precisely visit the performance modulation of functionalized separator in Li-S batteries via consecutive multiscale analysisWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-04-04Full publication date if available
- Authors
-
Zhangxiang Hao, Jie Chen, Xuekun Lu, Liqun Kang, Chun Tan, Ruoyu Xu, Lixia Yuan, Dan J. L. Brett, Paul R. Shearing, Feng Ryan Wang, Yunhui HuangList of authors in order
- Landing page
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https://doi.org/10.1016/j.ensm.2022.04.003Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1016/j.ensm.2022.04.003Direct OA link when available
- Concepts
-
Separator (oil production), Materials science, Polysulfide, X-ray absorption fine structure, Doping, Chemical engineering, Nanotechnology, Optoelectronics, Physical chemistry, Electrode, Chemistry, Thermodynamics, Spectroscopy, Engineering, Physics, Quantum mechanics, ElectrolyteTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
15Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 5, 2024: 3, 2023: 5, 2022: 2Per-year citation counts (last 5 years)
- References (count)
-
42Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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