Preparation and Performance of Radiata-Pine-Derived Polyvinyl Alcohol/Carbon Quantum Dots Fluorescent Films Article Swipe
Li Xu
,
Yushu Zhang
,
Haiqing Pan
,
Nan Xu
,
Changtong Mei
,
Haiyan Mao
,
Wenqing Zhang
,
Jiabin Cai
,
Changyan Xu
·
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.3390/ma13010067
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.3390/ma13010067
In this study, the low-cost processing residue of Radiata pine (Pinus radiata D. Don) was used as the lone carbon source for synthesis of CQDs (Carbon quantum dots) with a QY (The quantum yield of the CQDs) of 1.60%. The CQDs were obtained by the hydrothermal method, and +a PVA-based biofilm was prepared by the fluidized drying method. The effects of CQDs and CNF (cellulose nanofibers) content on the morphology, optical, mechanical, water-resistance, and wettability properties of the PVA/CQDs and PVA/CNF/CQDs films are discussed. The results revealed that, when the excitation wavelength was increased from 340 to 390 nm, the emission peak became slightly red-shifted, which was induced by the condensation between CQDs and PVA. The PVA composite films showed an increase in fluorescence intensity with the addition of the CNF and CQDs to polymers. The chemical structure of prepared films was determined by the FTIR spectroscopy, and no new chemical bonds were formed. In addition, the UV transmittance was inversely proportional to the change of CQDs content, which indicated that CQDs improved the UV barrier properties of the films. Furthermore, embedding CQDs Nano-materials and CNF into the PVA matrix improved the mechanical behavior of the Nano-composite. Tensile modulus and strength at break increased significantly with increasing the concentration of CQDs Nano-materials inside the Nano-composite, which was due to the increased in the density of crosslinking behavior. With the increase of CQDs content (>1 mL), the water absorption and surface contact angle of the prepared films decreased gradually, and the water-resistance and surface wettability of the films were improved. Therefore, PVA/CNF/CQDs bio-nanocomposite films could be used to prepare anti-counterfeiting, high-transparency, and ultraviolet-resistant composites, which have potential applications in ecological packaging materials.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/ma13010067
- https://www.mdpi.com/1996-1944/13/1/67/pdf?version=1577358169
- OA Status
- gold
- Cited By
- 73
- References
- 87
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2996293354
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W2996293354Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.3390/ma13010067Digital Object Identifier
- Title
-
Preparation and Performance of Radiata-Pine-Derived Polyvinyl Alcohol/Carbon Quantum Dots Fluorescent FilmsWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2019Year of publication
- Publication date
-
2019-12-21Full publication date if available
- Authors
-
Li Xu, Yushu Zhang, Haiqing Pan, Nan Xu, Changtong Mei, Haiyan Mao, Wenqing Zhang, Jiabin Cai, Changyan XuList of authors in order
- Landing page
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https://doi.org/10.3390/ma13010067Publisher landing page
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https://www.mdpi.com/1996-1944/13/1/67/pdf?version=1577358169Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.mdpi.com/1996-1944/13/1/67/pdf?version=1577358169Direct OA link when available
- Concepts
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Polyvinyl alcohol, Fluorescence, Radiata, Carbon quantum dots, Quantum dot, Materials science, Carbon fibers, Chemical engineering, Nanotechnology, Photochemistry, Composite material, Chemistry, Optics, Physics, Botany, Composite number, Biology, Vigna, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
73Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 22, 2024: 11, 2023: 6, 2022: 10, 2021: 17Per-year citation counts (last 5 years)
- References (count)
-
87Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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