Preparation of visible-light active MOFs-Perovskites (ZIF-67/LaFeO3) nanocatalysts for exceptional CO2 conversion, organic pollutants and antibiotics degradation Article Swipe

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Aftab Khan , Samreen Sadiq , Iltaf Khan , Muhammad Humayun , Jiyuan Guo , Muhammad Usman , Abbas Khan , Shoaib Khan , Amal Faleh Alanazi , M. Bououdina ·

YOU? · · 2024 · Open Access · · DOI: https://doi.org/10.1016/j.heliyon.2024.e27378

Modern industries rapid expansion has heightened energy needs and accelerated fossil fuel depletion, contributing to global warming. Additionally, organic pollutants present substantial risks to aquatic ecosystems due to their stability, insolubility, and non-biodegradability. Scientists are currently researching high-performance materials to address these issues. LaFeO₃ nanosheets (LFO-NS) were synthesized in this study using a solvothermal method with polyvinylpyrrolidone (PVP) as a soft template. The LFO-NS demonstrate superior performance, large surface area and charge separation than that of LaFeO₃ nanoparticles (LFO-NP). The LFO-NS performance is further upgraded by incorporating ZIF-67. Our results confirmed the ZIF-67/LFO-NS nanocomposite have superior performances than pure LFO-NP and ZIF-67. The integration of ZIF-67 has enhanced the charge separation and promote the surface area of LFO-NSwhich was confirmed by various characterization techniques including TEM, HRTEM, DRS, EDX, XRD, FS, XPS, FT-IR, BET, PL, and RAMAN. The 5ZIF-67/LFO-NS sample showed significant activities for CO₂ conversion, malachite green degradation, and antibiotics (cefazolin, oxacillin, and vancomycin) degradation. Furthermore, stability tests have confirmed that our optimal sample very active and stable. Furthermore, based on scavenger experiments and the photocatalytic degradation pathways, it has been established that H⁺ and •O₂^- are vital in the decomposition of MG and antibiotics. Our research work will open new gateways to prepare MOFs-Perovskites nanocatalysts for exceptional CO₂ conversion, organic pollutants and antibiotics degradation.

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Nanomaterial-based catalyst Materials science Chemical engineering Degradation (telecommunications) Nanotechnology Nanoparticle Engineering Computer science Telecommunications

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Type: article
Language: en
Landing Page: https://doi.org/10.1016/j.heliyon.2024.e27378
PDF: http://www.cell.com/article/S2405844024034091/pdf
OA Status: gold
Cited By: 42
References: 76
Related Works: 10
OpenAlex ID: https://openalex.org/W4392368659

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DOI: https://doi.org/10.1016/j.heliyon.2024.e27378

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Title: Preparation of visible-light active MOFs-Perovskites (ZIF-67/LaFeO3) nanocatalysts for exceptional CO2 conversion, organic pollutants and antibiotics degradation

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Type: article

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Language: en

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Publication year: 2024

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Publication date: 2024-03-01

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Authors: Aftab Khan, Samreen Sadiq, Iltaf Khan, Muhammad Humayun, Jiyuan Guo, Muhammad Usman, Abbas Khan, Shoaib Khan, Amal Faleh Alanazi, M. Bououdina

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Landing page: https://doi.org/10.1016/j.heliyon.2024.e27378

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PDF URL: https://www.cell.com/article/S2405844024034091/pdf

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Concepts: Nanomaterial-based catalyst, Materials science, Chemical engineering, Degradation (telecommunications), Nanotechnology, Nanoparticle, Engineering, Computer science, Telecommunications

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Cited by: 42

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