Pressure induced transition from chiral charge order to time-reversal symmetry-breaking superconducting state in Nb-doped CsV3Sb5 Article Swipe

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J. N. Graham , S. S. Islam , V. Sazgari , Y. Li , Hanbin Deng , Gianluca Janka , Yigui Zhong , O. Gerguri , P. Král , Andrin Doll , I. Biało , J. Chang , Z. Salman , Andreas Suter , T. Prokscha , Yugui Yao , Kozo Okazaki , H. Luetkens , R. Khasanov , Zhiwei Wang , Jia‐Xin Yin , Zurab Guguchia ·

YOU? · · 2025 · Open Access · · DOI: https://doi.org/10.1038/s42005-025-02235-6

Understanding how time-reversal symmetry (TRS) breaks in quantum materials is key to uncovering new states of matter and advancing quantum technologies. However, unraveling the interplay between TRS breaking, charge order, and superconductivity in kagome metals continues to be a compelling challenge. Here, we investigate the kagome metal Cs(V_1-x Nb _x )₃Sb₅ with x = 0.07 using muon spin rotation (μSR), alternating current (AC) magnetic susceptibility, and scanning tunneling microscopy (STM), under combined tuning by chemical doping, hydrostatic pressure, magnetic field, and depth from the surface. We find that TRS breaking in the bulk emerges below 40 K-lower than the charge order onset at 58 K-while near the surface, TRS breaking onsets at 58 K and is twice as strong. Niobium doping raises the superconducting critical temperature from 2.5 K to 4.4 K. Under pressure, both the critical temperature and superfluid density double, with TRS-breaking superconductivity appearing above 0.85 GPa. These findings reveal a depth-tunable TRS-breaking state and unconventional superconducting behavior in kagome systems.

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Superconductivity

Condensed Matter Physics

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Superconductivity Condensed matter physics Charge (physics) Doping T-symmetry Symmetry (geometry) State (computer science) Symmetry breaking Physics Order (exchange) Materials science Quantum mechanics Mathematics Geometry Algorithm Economics Finance

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Type: article
Language: en
Landing Page: https://doi.org/10.1038/s42005-025-02235-6
PDF: https://www.nature.com/articles/s42005-025-02235-6.pdf
OA Status: gold
Cited By: 1
References: 56
Related Works: 10
OpenAlex ID: https://openalex.org/W4412860197

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DOI: https://doi.org/10.1038/s42005-025-02235-6

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Title: Pressure induced transition from chiral charge order to time-reversal symmetry-breaking superconducting state in Nb-doped CsV3Sb5

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Type: article

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Language: en

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Publication year: 2025

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Publication date: 2025-08-02

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Authors: J. N. Graham, S. S. Islam, V. Sazgari, Y. Li, Hanbin Deng, Gianluca Janka, Yigui Zhong, O. Gerguri, P. Král, Andrin Doll, I. Biało, J. Chang, Z. Salman, Andreas Suter, T. Prokscha, Yugui Yao, Kozo Okazaki, H. Luetkens, R. Khasanov, Zhiwei Wang, Jia‐Xin Yin, Zurab Guguchia

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Landing page: https://doi.org/10.1038/s42005-025-02235-6

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Concepts: Superconductivity, Condensed matter physics, Charge (physics), Doping, T-symmetry, Symmetry (geometry), State (computer science), Symmetry breaking, Physics, Order (exchange), Materials science, Quantum mechanics, Mathematics, Geometry, Algorithm, Economics, Finance

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abstract_inverted_index.investigate	43
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abstract_inverted_index.TRS-breaking	143, 154
abstract_inverted_index.Understanding	0
abstract_inverted_index.depth-tunable	153
abstract_inverted_index.technologies.	20
abstract_inverted_index.time-reversal	2
abstract_inverted_index.(<i>μ</i>SR),	59
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abstract_inverted_index.Cs(V<sub>1-<i>x</i></sub>	47
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countries_distinct_count	4
institutions_distinct_count	22
sustainable_development_goals[0].id	https://metadata.un.org/sdg/13
sustainable_development_goals[0].score	0.5600000023841858
sustainable_development_goals[0].display_name	Climate action
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citation_normalized_percentile.is_in_top_10_percent	True