Programming Covalent Organic Frameworks for Photocatalysis: Investigation of Synthesis Methods Article Swipe
Wenbo Dong
,
Tianhua He
,
Longyu Li
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/chem.202500318
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/chem.202500318
Covalent organic frameworks (COFs) are crystalline, porous materials with exceptional potential as high‐performance photocatalysts for applications such as hydrogen and hydrogen peroxide production. In this study, we systematically evaluates various synthesis methods to optimize the preparation of COFs, specifically targeting enhanced photocatalytic activity. Four different synthetic strategies including solvothermal synthesis, microwave synthesis, ultrasonic synthesis, and mechanochemical synthesis were explored to prepare TAPT‐COF with identical molecular structures. Although all methods produced COFs with comparable crystallinity, porosity, and light absorption capacity, their photocatalytic efficiencies in hydrogen and hydrogen peroxide production varied significantly. Notably, the mechanochemical method, which involves ball milling to disrupt interlayer interactions and produce COF nanosheets, exhibited the highest photocatalytic performance, particularly in the COF‐BM‐30 min sample. This difference highlights the importance of morphology in photocatalytic activity. Our findings shed light on the impact of synthesis methods on COF properties and provide valuable guidance for molecular strategy development and industrial applications in photocatalysis.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/chem.202500318
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/chem.202500318
- OA Status
- bronze
- References
- 52
- Related Works
- 10
- OpenAlex ID
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Raw OpenAlex JSON
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https://doi.org/10.1002/chem.202500318Digital Object Identifier
- Title
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Programming Covalent Organic Frameworks for Photocatalysis: Investigation of Synthesis MethodsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-03-12Full publication date if available
- Authors
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Wenbo Dong, Tianhua He, Longyu LiList of authors in order
- Landing page
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https://doi.org/10.1002/chem.202500318Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/chem.202500318Direct link to full text PDF
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/chem.202500318Direct OA link when available
- Concepts
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Photocatalysis, Materials science, Hydrogen peroxide, Crystallinity, Covalent bond, Porosity, Nanotechnology, Chemical engineering, Ball mill, Catalysis, Organic chemistry, Composite material, Chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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52Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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