Proximity-Induced Exchange Interaction and Prolonged Valley Lifetime in MoSe2/CrSBr Van-Der-Waals Heterostructure with Orthogonal Spin Textures Article Swipe
Andreas Beer
,
Klaus Zollner
,
Caique Serati de Brito
,
Paulo E. Faria
,
Philipp Parzefall
,
Talieh S. Ghiasi
,
Josep Ingla‐Aynés
,
Samuel Mañas‐Valero
,
Carla Boix‐Constant
,
Kenji Watanabe
,
Takashi Taniguchi
,
Jaroslav Fabian
,
Herre S. J. van der Zant
,
Y. Galvão Gobato
,
Christian Schüller
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1021/acsnano.4c07336
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1021/acsnano.4c07336
Heterostructures, composed of semiconducting transition-metal dichalcogenides (TMDC) and magnetic van-der-Waals materials, offer exciting prospects for the manipulation of the TMDC valley properties via proximity interaction with the magnetic material. We show that the atomic proximity of monolayer MoSe2 and the antiferromagnetic van-der-Waals crystal CrSBr leads to an unexpected breaking of time-reversal symmetry, with originally perpendicular spin directions in both materials. The observed effect can be traced back to a proximity-induced exchange interaction via first-principles calculations. The resulting spin splitting in MoSe2 is determined experimentally and theoretically to be on the order of a few meV. Moreover, we find a more than 2 orders of magnitude longer valley lifetime of spin-polarized charge carriers in the heterostructure, as compared to monolayer MoSe2/SiO2, driven by a Mott transition in the type-III band-aligned heterostructure.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acsnano.4c07336
- OA Status
- hybrid
- Cited By
- 8
- References
- 80
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4403828309
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4403828309Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1021/acsnano.4c07336Digital Object Identifier
- Title
-
Proximity-Induced Exchange Interaction and Prolonged Valley Lifetime in MoSe2/CrSBr Van-Der-Waals Heterostructure with Orthogonal Spin TexturesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-10-28Full publication date if available
- Authors
-
Andreas Beer, Klaus Zollner, Caique Serati de Brito, Paulo E. Faria, Philipp Parzefall, Talieh S. Ghiasi, Josep Ingla‐Aynés, Samuel Mañas‐Valero, Carla Boix‐Constant, Kenji Watanabe, Takashi Taniguchi, Jaroslav Fabian, Herre S. J. van der Zant, Y. Galvão Gobato, Christian SchüllerList of authors in order
- Landing page
-
https://doi.org/10.1021/acsnano.4c07336Publisher landing page
- Open access
-
YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
- OA URL
-
https://doi.org/10.1021/acsnano.4c07336Direct OA link when available
- Concepts
-
van der Waals force, Materials science, Spin (aerodynamics), Heterojunction, Condensed matter physics, Exchange interaction, Chemical physics, Nanotechnology, Chemistry, Ferromagnetism, Physics, Molecule, Quantum mechanics, ThermodynamicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
8Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 8Per-year citation counts (last 5 years)
- References (count)
-
80Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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