Quantifying Interface‐Performance Relationships in Electrochemical CO2 Reduction through Mixed‐Dimensional Assembly of Nanocrystal‐on‐Nanowire Superstructures Article Swipe
Hushui Chen
,
Taishi Xiao
,
Yan Xia
,
Hengyao Song
,
Xiangyun Xi
,
Xianwu Huang
,
Dong Yang
,
Tongtao Li
,
Zhengzong Sun
,
Angang Dong
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202410039
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202410039
Fine‐tuning the interfacial sites within heterogeneous catalysts is pivotal for unravelling the intricate structure–property relationship and optimizing their catalytic performance. Herein, a simple and versatile mixed‐dimensional assembly approach is proposed to create nanocrystal‐on‐nanowire superstructures with precisely adjustable numbers of biphasic interfaces. This method leverages an efficient self‐assembly process in which colloidal nanocrystals spontaneously organize onto Ag nanowires, driven by the solvophobic effect. Importantly, varying the ratio of the two components during assembly allows for accurate control over both the quantity and contact perimeter of biphasic interfaces. As a proof‐of‐concept demonstration, a series of Au‐on‐Ag superstructures with varying numbers of Au/Ag interfaces are constructed and employed as electrocatalysts for electrochemical CO 2 ‐to‐CO conversion. Experimental results reveal a logarithmic linear relationship between catalytic activity and the number of Au/Ag interfaces per unit mass of Au‐on‐Ag superstructures. This work presents a straightforward approach for precise interface engineering, paving the way for systematic exploration of interface‐dependent catalytic behaviors in heterogeneous catalysts.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/ange.202410039
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/ange.202410039
- OA Status
- bronze
- References
- 63
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4402019542
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4402019542Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/ange.202410039Digital Object Identifier
- Title
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Quantifying Interface‐Performance Relationships in Electrochemical CO2 Reduction through Mixed‐Dimensional Assembly of Nanocrystal‐on‐Nanowire SuperstructuresWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-08-29Full publication date if available
- Authors
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Hushui Chen, Taishi Xiao, Yan Xia, Hengyao Song, Xiangyun Xi, Xianwu Huang, Dong Yang, Tongtao Li, Zhengzong Sun, Angang DongList of authors in order
- Landing page
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https://doi.org/10.1002/ange.202410039Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/ange.202410039Direct link to full text PDF
- Open access
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/ange.202410039Direct OA link when available
- Concepts
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Nanocrystal, Nanowire, Materials science, Electrochemistry, Nanotechnology, Interface (matter), Reduction (mathematics), Chemistry, Electrode, Physical chemistry, Composite material, Mathematics, Geometry, Capillary action, Capillary numberTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- References (count)
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63Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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