Rapid-scan nonlinear time-resolved spectroscopy over arbitrary delay intervals Article Swipe
Tobias Flöry
,
Vinzenz Stummer
,
Justinas Pupeikis
,
Benjamin Willenberg
,
Alexander Nussbaum-Lapping
,
Franco V. A. Camargo
,
Martynas Barkauskas
,
C. R. Phillips
,
U. Keller
,
Giulio Cerullo
,
A. Pugžlys
,
Andrius Baltuška
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2211.12211
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2211.12211
Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this technique found already application for nonlinear time-resolved spectroscopy within the energy limit available from sources operating at the full oscillator repetition rate. Here, we present a technique based on time filtering of femtosecond frequency combs by pulse gating in a laser amplifier. This gives the required boost to the pulse energy and provides the flexibility to engineer pairs of arbitrarily delayed wavelength-tunable pulses for pump-probe techniques. Using a dual-channel millijoule amplifier, we demonstrate programmable generation of both extremely short, fs, and extremely long (>ns) interpulse delays. A predetermined arbitrarily chosen interpulse delay can be directly realized in each successive amplifier shot, eliminating the massive waiting time required to alter the delay setting by means of an optomechanical line or an asynchronous scan of two free-running oscillators. We confirm the versatility of this delay generation method by measuring chi^(2) cross-correlation and chi^(3) multicomponent population recovery kinetics.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://hdl.handle.net/20.500.11850/649384
- OA Status
- green
- Cited By
- 1
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4309873557
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4309873557Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2211.12211Digital Object Identifier
- Title
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Rapid-scan nonlinear time-resolved spectroscopy over arbitrary delay intervalsWork title
- Type
-
preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-11-22Full publication date if available
- Authors
-
Tobias Flöry, Vinzenz Stummer, Justinas Pupeikis, Benjamin Willenberg, Alexander Nussbaum-Lapping, Franco V. A. Camargo, Martynas Barkauskas, C. R. Phillips, U. Keller, Giulio Cerullo, A. Pugžlys, Andrius BaltuškaList of authors in order
- Landing page
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https://hdl.handle.net/20.500.11850/649384Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://hdl.handle.net/20.500.11850/649384Direct OA link when available
- Concepts
-
Femtosecond, Laser, Optics, Amplifier, Time domain, Physics, Spectroscopy, Computer science, Optoelectronics, CMOS, Quantum mechanics, Computer visionTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
1Total citation count in OpenAlex
- Citations by year (recent)
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2023: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| primary_location.raw_source_name | Ultrafast Science, 3 |
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| publication_year | 2022 |
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