Reaction performance in T-, X- and arrow-shaped microdevices Article Swipe
Sara Tomasi Masoni
,
Alessandro Mariotti
,
Matteo Antognoli
,
Chiara Galletti
,
Roberto Mauri
,
Maria Vittoria Salvetti
,
Elisabetta Brunazzi
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1016/j.cherd.2023.03.032
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1016/j.cherd.2023.03.032
Microreactors are widely used for continuous flow operations. The assessment of their performance has a crucial role in determining the optimal geometries and working con-ditions. Among the most common geometries, we compare T-, X-and arrow-shaped de-vices to highlight how flow features, mixing degree and residence time affect the reaction yield and productivity. We focus on the steady flow regimes occurring in the three devices fed with reactive streams for varying Reynolds numbers. The Reynolds number, Rei, is herein based on the bulk velocity and the inlet-channel hydraulic diameter. The flow regimes presenting a central vortex in the mixing channel, found in X-and arrow-mi-croreactors, lead to the best mixing and reaction yield. For Rei <= 120 the maximum pro-ductivity is obtained with the X-microreactor, whereas above Rei = 120, with the arrow-reactor. Conversely, lower reaction yields and productivities are found in the T-micro-reactor, which exhibits an engulfment regime with two co-rotating vortices in the mixing channel. It is thus evident that the spiral pattern induced by a single central vortex ex-tends the contact area between the reactants and leads to better performance. In terms of reaction cost, for the lower productivity values, the associated pressure drops are similar for all three geometries. For higher productivities, the best performance, i.e., the lowest pressure drops, is reached in the arrow-microreactor, followed by the T-and, then, by the X-device.(c) 2023 Institution of Chemical Engineers. Published by Elsevier Ltd. All rights reserved.
Related Topics
Concepts
Microreactor
Reynolds number
Mixing (physics)
Yield (engineering)
Mechanics
Vortex
Flow (mathematics)
Materials science
Residence time (fluid dynamics)
Pressure drop
Thermodynamics
Chemistry
Physics
Turbulence
Engineering
Composite material
Catalysis
Biochemistry
Geotechnical engineering
Quantum mechanics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.cherd.2023.03.032
- OA Status
- hybrid
- Cited By
- 4
- References
- 34
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4353099902
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4353099902Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.cherd.2023.03.032Digital Object Identifier
- Title
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Reaction performance in T-, X- and arrow-shaped microdevicesWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-03-22Full publication date if available
- Authors
-
Sara Tomasi Masoni, Alessandro Mariotti, Matteo Antognoli, Chiara Galletti, Roberto Mauri, Maria Vittoria Salvetti, Elisabetta BrunazziList of authors in order
- Landing page
-
https://doi.org/10.1016/j.cherd.2023.03.032Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1016/j.cherd.2023.03.032Direct OA link when available
- Concepts
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Microreactor, Reynolds number, Mixing (physics), Yield (engineering), Mechanics, Vortex, Flow (mathematics), Materials science, Residence time (fluid dynamics), Pressure drop, Thermodynamics, Chemistry, Physics, Turbulence, Engineering, Composite material, Catalysis, Biochemistry, Geotechnical engineering, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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4Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 1Per-year citation counts (last 5 years)
- References (count)
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34Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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