Realizing Two-Dimensional Supramolecular Arrays of a Spin Molecule via Halogen Bonding Article Swipe
Dingguan Wang
,
Zishen Wang
,
Shaofei Wu
,
Arramel Arramel
,
Xinmao Yin
,
Chi Sin Tang
,
Yuan Ping Feng
,
Jishan Wu
,
Andrew T. S. Wee
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acsnanoscienceau.2c00005
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acsnanoscienceau.2c00005
Well-ordered spin arrays are desirable for next-generation molecule-based magnetic devices, yet their synthetic method remains a challenging task. Herein, we demonstrate the realization of two-dimensional supramolecular spin arrays on surfaces via halogen-bonding molecular self-assembly. A bromine-terminated perchlorotriphenylmethyl radical with net carbon spin was synthesized and deposited on Au(111) to achieve two-dimensional supramolecular spin arrays. By taking advantage of the diversity of halogen bonds, five supramolecular spin arrays form and are probed by low-temperature scanning tunneling microscopy at the single-molecule level. First-principles calculations verify that the formation of three distinct types of halogen bonds can be used to tailor supramolecular spin arrays via molecular coverage and annealing temperature. Our work suggests that supramolecular self-assembly can be a promising method to engineer two-dimensional molecular spin arrays.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acsnanoscienceau.2c00005
- OA Status
- gold
- Cited By
- 2
- References
- 59
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4225374883
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4225374883Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1021/acsnanoscienceau.2c00005Digital Object Identifier
- Title
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Realizing Two-Dimensional Supramolecular Arrays of a Spin Molecule via Halogen BondingWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
-
2022-05-03Full publication date if available
- Authors
-
Dingguan Wang, Zishen Wang, Shaofei Wu, Arramel Arramel, Xinmao Yin, Chi Sin Tang, Yuan Ping Feng, Jishan Wu, Andrew T. S. WeeList of authors in order
- Landing page
-
https://doi.org/10.1021/acsnanoscienceau.2c00005Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://doi.org/10.1021/acsnanoscienceau.2c00005Direct OA link when available
- Concepts
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Supramolecular chemistry, Halogen bond, Materials science, Molecule, Supramolecular assembly, Scanning tunneling microscope, Nanotechnology, Halogen, Spin (aerodynamics), Chemical physics, Crystallography, Chemistry, Hydrogen bond, Physics, Organic chemistry, Alkyl, ThermodynamicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
2Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 2Per-year citation counts (last 5 years)
- References (count)
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59Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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