Removal of Hemicellulose from Alkaline Lignin Improved Electrochemical Performance of Hard Carbon for Sodium-Ion Battery Application Article Swipe
Nethmi Kulanika Dayarathne
,
Eric Campbell
,
Mansi Goyal
,
Mu Xiao
,
Xueping Song
,
Cheng Yan
,
Hongxia Wang
,
Dawei Wang
,
Yu Lin Zhong
,
Zhanying Zhang
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1088/2752-5724/ae1522
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1088/2752-5724/ae1522
Lignin, a natural aromatic biopolymer, is often recovered as low-value by-product during the delignification process of lignocellulosic biomass for producing cellulosic pulps. In this study, crude alkaline lignin (CAL) derived from the NaOH-pretreated sugarcane bagasse was used to produce hard carbon (HC) for sodium-ion battery (SIB) anode applications. The results showed that the direct use of CAL led to HC with a maximum initial coulombic efficiency (ICE) and reversible capacity of only 60.2% and 198.5 mAh g-1 respectively. To improve the electrochemical performance, solvent extraction was applied to purify CAL. The use of purified alkaline lignin (PAL) led to HC with a maximum ICE of 76.1% and reversible capacity of 277.5 mAh g-1, which were significantly higher than CAL-derived HC. The effects of carbonization temperature (1200–1400 °C) and heating rate (1–8 °C min-1) were also examined. Structural analyses revealed that hemicellulose removal resulted in HC with favorable microstructural structures, including short-range graphitic layers, closed pores, and reduced defects, facilitating the storage of Na ions. Additionally, the overall yield of PAL-HC was comparable to CAL-HC. These results demonstrated that the removal of hemicellulose is a critical initial step towards improving the electrochemical performance of HC prior to the application of other strategies.
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Removal of Hemicellulose from Alkaline Lignin Improved Electrochemical Performance of Hard Carbon for Sodium-Ion Battery ApplicationWork title
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articleOpenAlex work type
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2025Year of publication
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2025-10-20Full publication date if available
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Nethmi Kulanika Dayarathne, Eric Campbell, Mansi Goyal, Mu Xiao, Xueping Song, Cheng Yan, Hongxia Wang, Dawei Wang, Yu Lin Zhong, Zhanying ZhangList of authors in order
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https://doi.org/10.1088/2752-5724/ae1522Publisher landing page
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diamondOpen access status per OpenAlex
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https://doi.org/10.1088/2752-5724/ae1522Direct OA link when available
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| abstract_inverted_index.this | 24 |
| abstract_inverted_index.used | 37 |
| abstract_inverted_index.were | 115, 134 |
| abstract_inverted_index.with | 61, 101, 146 |
| abstract_inverted_index.°C) | 127 |
| abstract_inverted_index.(CAL) | 29 |
| abstract_inverted_index.(ICE) | 67 |
| abstract_inverted_index.(PAL) | 97 |
| abstract_inverted_index.(SIB) | 46 |
| abstract_inverted_index.198.5 | 75 |
| abstract_inverted_index.277.5 | 111 |
| abstract_inverted_index.60.2% | 73 |
| abstract_inverted_index.76.1% | 106 |
| abstract_inverted_index.These | 175 |
| abstract_inverted_index.anode | 47 |
| abstract_inverted_index.crude | 26 |
| abstract_inverted_index.ions. | 164 |
| abstract_inverted_index.often | 7 |
| abstract_inverted_index.other | 200 |
| abstract_inverted_index.prior | 195 |
| abstract_inverted_index.which | 114 |
| abstract_inverted_index.yield | 168 |
| abstract_inverted_index.(1–8 | 131 |
| abstract_inverted_index.PAL-HC | 170 |
| abstract_inverted_index.carbon | 41 |
| abstract_inverted_index.closed | 154 |
| abstract_inverted_index.direct | 54 |
| abstract_inverted_index.during | 12 |
| abstract_inverted_index.higher | 117 |
| abstract_inverted_index.lignin | 28, 96 |
| abstract_inverted_index.min-1) | 133 |
| abstract_inverted_index.pores, | 155 |
| abstract_inverted_index.pulps. | 22 |
| abstract_inverted_index.purify | 89 |
| abstract_inverted_index.showed | 51 |
| abstract_inverted_index.study, | 25 |
| abstract_inverted_index.CAL-HC. | 174 |
| abstract_inverted_index.Lignin, | 1 |
| abstract_inverted_index.applied | 87 |
| abstract_inverted_index.bagasse | 35 |
| abstract_inverted_index.battery | 45 |
| abstract_inverted_index.biomass | 18 |
| abstract_inverted_index.derived | 30 |
| abstract_inverted_index.effects | 122 |
| abstract_inverted_index.heating | 129 |
| abstract_inverted_index.improve | 80 |
| abstract_inverted_index.initial | 64, 186 |
| abstract_inverted_index.layers, | 153 |
| abstract_inverted_index.maximum | 63, 103 |
| abstract_inverted_index.natural | 3 |
| abstract_inverted_index.overall | 167 |
| abstract_inverted_index.process | 15 |
| abstract_inverted_index.produce | 39 |
| abstract_inverted_index.reduced | 157 |
| abstract_inverted_index.removal | 142, 180 |
| abstract_inverted_index.results | 50, 176 |
| abstract_inverted_index.solvent | 84 |
| abstract_inverted_index.storage | 161 |
| abstract_inverted_index.towards | 188 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.alkaline | 27, 95 |
| abstract_inverted_index.analyses | 138 |
| abstract_inverted_index.aromatic | 4 |
| abstract_inverted_index.capacity | 70, 109 |
| abstract_inverted_index.critical | 185 |
| abstract_inverted_index.defects, | 158 |
| abstract_inverted_index.purified | 94 |
| abstract_inverted_index.resulted | 143 |
| abstract_inverted_index.revealed | 139 |
| abstract_inverted_index.coulombic | 65 |
| abstract_inverted_index.examined. | 136 |
| abstract_inverted_index.favorable | 147 |
| abstract_inverted_index.graphitic | 152 |
| abstract_inverted_index.improving | 189 |
| abstract_inverted_index.including | 150 |
| abstract_inverted_index.low-value | 10 |
| abstract_inverted_index.producing | 20 |
| abstract_inverted_index.recovered | 8 |
| abstract_inverted_index.sugarcane | 34 |
| abstract_inverted_index.Structural | 137 |
| abstract_inverted_index.by-product | 11 |
| abstract_inverted_index.cellulosic | 21 |
| abstract_inverted_index.comparable | 172 |
| abstract_inverted_index.efficiency | 66 |
| abstract_inverted_index.extraction | 85 |
| abstract_inverted_index.reversible | 69, 108 |
| abstract_inverted_index.sodium-ion | 44 |
| abstract_inverted_index.CAL-derived | 119 |
| abstract_inverted_index.application | 198 |
| abstract_inverted_index.biopolymer, | 5 |
| abstract_inverted_index.performance | 192 |
| abstract_inverted_index.short-range | 151 |
| abstract_inverted_index.strategies. | 201 |
| abstract_inverted_index.structures, | 149 |
| abstract_inverted_index.temperature | 125 |
| abstract_inverted_index.(1200–1400 | 126 |
| abstract_inverted_index.demonstrated | 177 |
| abstract_inverted_index.facilitating | 159 |
| abstract_inverted_index.performance, | 83 |
| abstract_inverted_index.Additionally, | 165 |
| abstract_inverted_index.applications. | 48 |
| abstract_inverted_index.carbonization | 124 |
| abstract_inverted_index.hemicellulose | 141, 182 |
| abstract_inverted_index.respectively. | 78 |
| abstract_inverted_index.significantly | 116 |
| abstract_inverted_index.NaOH-pretreated | 33 |
| abstract_inverted_index.delignification | 14 |
| abstract_inverted_index.electrochemical | 82, 191 |
| abstract_inverted_index.lignocellulosic | 17 |
| abstract_inverted_index.microstructural | 148 |
| cited_by_percentile_year | |
| corresponding_author_ids | https://openalex.org/A5100445442, https://openalex.org/A5021226984, https://openalex.org/A5059990116, https://openalex.org/A5069298813, https://openalex.org/A5046353687, https://openalex.org/A5100378083, https://openalex.org/A5028493558, https://openalex.org/A5116874664, https://openalex.org/A5110739052, https://openalex.org/A5050425437 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 10 |
| corresponding_institution_ids | https://openalex.org/I11701301, https://openalex.org/I150807315, https://openalex.org/I160993911, https://openalex.org/I165143802, https://openalex.org/I180726961, https://openalex.org/I4210152380 |
| citation_normalized_percentile.value | 0.54788746 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |