Resonant inelastic x-ray scattering in the topological semimetal FeSi Article Swipe
YOU?
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· 2024
· Open Access
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· DOI: https://doi.org/10.1103/physrevb.110.245137
The energy spectrum of topological semimetals contains protected degeneracies in reciprocal space that correspond to Weyl, Dirac, or multifold fermionic states. To exploit the unconventional properties of these states, one has to access the electronic structure of the three-dimensional bulk. In this paper, we present a joint theory-experiment study of the electronic structure of a candidate topological semimetal with resonant inelastic x-ray scattering (RIXS). We resolve the bulk electronic states of FeSi using momentum-dependent RIXS at the Fe L3 edge. We observe a broad excitation continuum devoid of sharp features, consistent with particle-hole scattering in an underlying electronic band structure. Using density functional theory (DFT), we calculate the electronic structure of FeSi and derive a band theory formulation of RIXS in the fast collision approximation to model the scattering process with zero adjustable parameters. While band theory predicts an excitation continuum with broad spectral features similar to the observed ones, discrepancies between theory and experiment suggest the presence of low-energy processes that DFT alone does not account for. Further, this study of RIXS in a topological semimetal shows that RIXS is a useful tool for revealing unanticipated behavior of bulk electronic states in this class of materials.
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- article
- Language
- en
- Landing Page
- https://doi.org/10.1103/physrevb.110.245137
- OA Status
- green
- References
- 56
- Related Works
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- OpenAlex ID
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https://openalex.org/W4405736856Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1103/physrevb.110.245137Digital Object Identifier
- Title
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Resonant inelastic x-ray scattering in the topological semimetal FeSiWork title
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articleOpenAlex work type
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-12-24Full publication date if available
- Authors
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Yao Shen, Anirudh Chandrasekaran, Jennifer Sears, Tiantian Zhang, Xin Han, Youguo Shi, Jiemin Li, Jonathan Pelliciari, Valentina Bisogni, M. P. M. Dean, Stefanos KourtisList of authors in order
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https://doi.org/10.1103/physrevb.110.245137Publisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/2503921Direct OA link when available
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Icon, Physics, Scattering, Topology (electrical circuits), Resonant inelastic X-ray scattering, Electronic structure, Excitation, Condensed matter physics, Inelastic scattering, Quantum mechanics, Inelastic neutron scattering, Mathematics, Computer science, Programming language, CombinatoricsTop concepts (fields/topics) attached by OpenAlex
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10Other works algorithmically related by OpenAlex
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