Scalable Preparation of Polyzwitterionic Hydrogels Based on Hydration Shielding‐Accelerated Redox Self‐Catalytic Polymerization (HS‐A‐RP) Article Swipe
Renjie Li
,
Lunkun Liu
,
Yunlei Zhang
,
Weiyi Zhao
,
Xiaoduo Zhao
,
Ying Liu
,
Bo Yu
,
Shuanhong Ma
,
Feng Zhou
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202424129
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202424129
Traditional synthesis methods for polyzwitterionic hydrogels involve harsh conditions, such as thermal or UV irradiation, prolonged durations, and high monomer concentrations. Herein, we address these challenges at the meantime by proposing a novel chemical method, called hydration‐shielding accelerated self‐catalytic polymerization (HS‐A‐RP), facilitating the preparation of polyzwitterionic hydrogels. The discovery is that polyvinyl alcohol (PVA) chains can generate hydration shielding around hydrated zwitterionic monomers, promoting their effective aggregation and rapid crosslinking polymerization under the assistance of silver ions (Ag + )‐potassium persulfate (S 2 O 8 2‐ ) redox catalyst. The HS‐A‐RP method performs under mild condition (−5 °C to 37 °C) without extra energy, overcomes the critical monomer polymerization concentration limitation (wt%: 0.3%), and completes within an ultrashort polymerization time (<60 s). The prepared polyzwitterionic hydrogels possesses a denser network and superior mechanical properties compared to those prepared by traditional thermal/UV methods, exhibiting good antiswelling behavior, excellent lubrication performance, and significant antibacterial and anti‐fouling properties. These significant advances endow HS‐A‐RP with attractive application potentials in manufacturing functional hydrogel coatings for biomedical device, in situ encapsulation of thermally sensitive materials, and excellent sand fixation abilities. Moreover, HS‐A‐RP method is suitable for scalable manufacture and decorative coating of polyzwitterionic hydrogels on diverse substrates in extreme environmental conditions.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/anie.202424129
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202424129
- OA Status
- bronze
- Cited By
- 3
- References
- 38
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4409444051
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4409444051Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/anie.202424129Digital Object Identifier
- Title
-
Scalable Preparation of Polyzwitterionic Hydrogels Based on Hydration Shielding‐Accelerated Redox Self‐Catalytic Polymerization (HS‐A‐RP)Work title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-04-15Full publication date if available
- Authors
-
Renjie Li, Lunkun Liu, Yunlei Zhang, Weiyi Zhao, Xiaoduo Zhao, Ying Liu, Bo Yu, Shuanhong Ma, Feng ZhouList of authors in order
- Landing page
-
https://doi.org/10.1002/anie.202424129Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202424129Direct link to full text PDF
- Open access
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202424129Direct OA link when available
- Concepts
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Self-healing hydrogels, Polymerization, Monomer, Materials science, Potassium persulfate, Chemical engineering, Coating, Polyvinyl alcohol, Polymer chemistry, Nanotechnology, Polymer, Composite material, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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3Total citation count in OpenAlex
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2025: 3Per-year citation counts (last 5 years)
- References (count)
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38Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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