Self-assembly of nanocrystal checkerboard patterns via non-specific interactions Article Swipe
Yufei Wang
,
Yilong Zhou
,
Quanpeng Yang
,
Rourav Basak
,
Yu Xie
,
Dong Le
,
Alexander Fuqua
,
Wade Shipley
,
Zachary Yam
,
Alex Frañó
,
Gaurav Arya
,
Andrea R. Tao
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-024-47572-2
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-024-47572-2
Checkerboard lattices—where the resulting structure is open, porous, and highly symmetric—are difficult to create by self-assembly. Synthetic systems that adopt such structures typically rely on shape complementarity and site-specific chemical interactions that are only available to biomolecular systems (e.g., protein, DNA). Here we show the assembly of checkerboard lattices from colloidal nanocrystals that harness the effects of multiple, coupled physical forces at disparate length scales (interfacial, interparticle, and intermolecular) and that do not rely on chemical binding. Colloidal Ag nanocubes were bi-functionalized with mixtures of hydrophilic and hydrophobic surface ligands and subsequently assembled at an air–water interface. Using feedback between molecular dynamics simulations and interfacial assembly experiments, we achieve a periodic checkerboard mesostructure that represents a tiny fraction of the phase space associated with the polymer-grafted nanocrystals used in these experiments. In a broader context, this work expands our knowledge of non-specific nanocrystal interactions and presents a computation-guided strategy for designing self-assembling materials.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-024-47572-2
- https://www.nature.com/articles/s41467-024-47572-2.pdf
- OA Status
- gold
- Cited By
- 17
- References
- 29
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4396769426
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4396769426Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41467-024-47572-2Digital Object Identifier
- Title
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Self-assembly of nanocrystal checkerboard patterns via non-specific interactionsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-05-09Full publication date if available
- Authors
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Yufei Wang, Yilong Zhou, Quanpeng Yang, Rourav Basak, Yu Xie, Dong Le, Alexander Fuqua, Wade Shipley, Zachary Yam, Alex Frañó, Gaurav Arya, Andrea R. TaoList of authors in order
- Landing page
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https://doi.org/10.1038/s41467-024-47572-2Publisher landing page
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https://www.nature.com/articles/s41467-024-47572-2.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41467-024-47572-2.pdfDirect OA link when available
- Concepts
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Checkerboard, Nanocrystal, Nanotechnology, Self-assembly, Materials science, Biology, MicrobiologyTop concepts (fields/topics) attached by OpenAlex
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17Total citation count in OpenAlex
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2025: 13, 2024: 4Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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