Shining New Light on the Kinetics of Water Uptake by Organic Aerosol Particles Article Swipe
Matúš E. Divéky
,
Michael J. Gleichweit
,
Sandra Roy
,
Ruth Signorell
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpca.1c00202
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpca.1c00202
The uptake of water vapor by various organic aerosols is important in a number of applications ranging from medical delivery of pharmaceutical aerosols to cloud formation in the atmosphere. The coefficient that describes the probability that the impinging gas-phase molecule sticks to the surface of interest is called the mass accommodation coefficient, αM. Despite the importance of this coefficient for the description of water uptake kinetics, accurate values are still lacking for many systems. In this Feature Article, we present various experimental techniques that have been evoked in the literature to study the interfacial transport of water and discuss the corresponding strengths and limitations. This includes our recently developed technique called photothermal single-particle spectroscopy (PSPS). The PSPS technique allows for a retrieval of αM values from three independent, yet simultaneous measurements operating close to equilibrium, providing a robust assessment of interfacial mass transport. We review the currently available data for αM for water on various organics and discuss the few studies that address the temperature and relative humidity dependence of αM for water on organics. The knowledge of the latter, for example, is crucial to assess the water uptake kinetics of organic aerosols in the Earth's atmosphere. Finally, we argue that PSPS might also be a viable method to better restrict the αM value for water on liquid water.
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Metadata
- Type
- review
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.jpca.1c00202
- OA Status
- green
- Cited By
- 19
- References
- 231
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3139037475
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3139037475Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.jpca.1c00202Digital Object Identifier
- Title
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Shining New Light on the Kinetics of Water Uptake by Organic Aerosol ParticlesWork title
- Type
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reviewOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-03-19Full publication date if available
- Authors
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Matúš E. Divéky, Michael J. Gleichweit, Sandra Roy, Ruth SignorellList of authors in order
- Landing page
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https://doi.org/10.1021/acs.jpca.1c00202Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
- OA URL
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https://hdl.handle.net/20.500.11850/489168Direct OA link when available
- Concepts
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Aerosol, Kinetics, Environmental science, Environmental chemistry, Chemistry, Atmospheric sciences, Physics, Organic chemistry, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
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19Total citation count in OpenAlex
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2025: 2, 2024: 3, 2023: 8, 2022: 5, 2021: 1Per-year citation counts (last 5 years)
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231Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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