Simultaneous Observation of Carrier-Specific Redistribution and Coherent\n Lattice Dynamics in 2H-MoTe$_{2}$ with Femtosecond Core-Level Spectroscopy Article Swipe

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Andrew Attar , Hung-Tzu Chang , Alexander Britz , Xiang Zhang , Ming‐Fu Lin , Aravind Krishnamoorthy , Thomas Linker , David Fritz , Daniel M. Neumark , Rajiv K. Kalia , Aiichiro Nakano , Pulickel M. Ajayan , Priya Vashishta , Uwe Bergmann , Stephen R. Leone ·

YOU? · · 2020 · Open Access · · DOI: https://doi.org/10.48550/arxiv.2009.00721

We employ few-femtosecond extreme ultraviolet (XUV) transient absorption\nspectroscopy to reveal simultaneously the intra- and interband carrier\nrelaxation and the light-induced structural dynamics in nanoscale thin films of\nlayered 2H-MoTe$_{2}$ semiconductor. By interrogating the valence electronic\nstructure via localized Te 4$\\textit{d}$ (39-46 eV) and Mo 4$\\textit{p}$ (35-38\neV) core levels, the relaxation of the photoexcited hole distribution is\ndirectly observed in real time. We obtain hole thermalization and cooling times\nof 15$\\pm$5 fs and 380$\\pm$90 fs, respectively, and an electron-hole\nrecombination time of 1.5$\\pm$0.1 ps. Furthermore, excitations of coherent\nout-of-plane A$_{1g}$ (5.1 THz) and in-plane E$_{1g}$ (3.7 THz) lattice\nvibrations are visualized through oscillations in the XUV absorption spectra.\nBy comparison to Bethe-Salpeter equation simulations, the spectral changes are\nmapped to real-space excited-state displacements of the lattice along the\ndominant A$_{1g}$ coordinate. By directly and simultaneously probing the\nexcited carrier distribution dynamics and accompanying femtosecond lattice\ndisplacement in 2H-MoTe$_{2}$ within a single experiment, our work provides a\nbenchmark for understanding the interplay between electronic and structural\ndynamics in photoexcited nanomaterials.\n

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Femtosecond Excited state Spectroscopy Atomic physics Molecular physics Physics Ultrafast laser spectroscopy Extreme ultraviolet Absorption spectroscopy Materials science Lattice (music) Optics Laser Acoustics Quantum mechanics

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Type: preprint
Language: en
Landing Page: http://arxiv.org/abs/2009.00721
PDF: https://arxiv.org/pdf/2009.00721
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Title: Simultaneous Observation of Carrier-Specific Redistribution and Coherent\n Lattice Dynamics in 2H-MoTe$_{2}$ with Femtosecond Core-Level Spectroscopy

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Language: en

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Publication year: 2020

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Authors: Andrew Attar, Hung-Tzu Chang, Alexander Britz, Xiang Zhang, Ming‐Fu Lin, Aravind Krishnamoorthy, Thomas Linker, David Fritz, Daniel M. Neumark, Rajiv K. Kalia, Aiichiro Nakano, Pulickel M. Ajayan, Priya Vashishta, Uwe Bergmann, Stephen R. Leone

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Landing page: https://arxiv.org/abs/2009.00721

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Concepts: Femtosecond, Excited state, Spectroscopy, Atomic physics, Molecular physics, Physics, Ultrafast laser spectroscopy, Extreme ultraviolet, Absorption spectroscopy, Materials science, Lattice (music), Optics, Laser, Acoustics, Quantum mechanics

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abstract_inverted_index.in-plane	85
abstract_inverted_index.observed	53
abstract_inverted_index.provides	140
abstract_inverted_index.spectral	105
abstract_inverted_index.15$\\pm$5	64
abstract_inverted_index.interband	14
abstract_inverted_index.interplay	145
abstract_inverted_index.localized	34
abstract_inverted_index.nanoscale	22
abstract_inverted_index.times\nof	63
abstract_inverted_index.transient	6
abstract_inverted_index.absorption	97
abstract_inverted_index.comparison	99
abstract_inverted_index.electronic	147
abstract_inverted_index.real-space	109
abstract_inverted_index.relaxation	46
abstract_inverted_index.structural	19
abstract_inverted_index.visualized	91
abstract_inverted_index.(35-38\neV)	42
abstract_inverted_index.380$\\pm$90	67
abstract_inverted_index.are\nmapped	107
abstract_inverted_index.coordinate.	118
abstract_inverted_index.excitations	78
abstract_inverted_index.experiment,	137
abstract_inverted_index.femtosecond	130
abstract_inverted_index.of\nlayered	25
abstract_inverted_index.ultraviolet	4
abstract_inverted_index.1.5$\\pm$0.1	75
abstract_inverted_index.Furthermore,	77
abstract_inverted_index.a\nbenchmark	141
abstract_inverted_index.accompanying	129
abstract_inverted_index.distribution	51, 126
abstract_inverted_index.is\ndirectly	52
abstract_inverted_index.oscillations	93
abstract_inverted_index.photoexcited	49, 151
abstract_inverted_index.simulations,	103
abstract_inverted_index.spectra.\nBy	98
abstract_inverted_index.the\nexcited	124
abstract_inverted_index.2H-MoTe$_{2}$	26, 133
abstract_inverted_index.displacements	111
abstract_inverted_index.excited-state	110
abstract_inverted_index.interrogating	29
abstract_inverted_index.light-induced	18
abstract_inverted_index.respectively,	69
abstract_inverted_index.the\ndominant	116
abstract_inverted_index.understanding	143
abstract_inverted_index.4$\\textit{d}$	36
abstract_inverted_index.4$\\textit{p}$	41
abstract_inverted_index.Bethe-Salpeter	101
abstract_inverted_index.semiconductor.	27
abstract_inverted_index.simultaneously	10, 122
abstract_inverted_index.thermalization	60
abstract_inverted_index.few-femtosecond	2
abstract_inverted_index.nanomaterials.\n	152
abstract_inverted_index.carrier\nrelaxation	15
abstract_inverted_index.lattice\nvibrations	89
abstract_inverted_index.structural\ndynamics	149
abstract_inverted_index.electronic\nstructure	32
abstract_inverted_index.lattice\ndisplacement	131
abstract_inverted_index.coherent\nout-of-plane	80
abstract_inverted_index.absorption\nspectroscopy	7
abstract_inverted_index.electron-hole\nrecombination	72
cited_by_percentile_year
countries_distinct_count	0
institutions_distinct_count	15
citation_normalized_percentile.value	0.22876324
citation_normalized_percentile.is_in_top_1_percent	False
citation_normalized_percentile.is_in_top_10_percent	False