Small polarons mediated near-room-temperature metal-insulator transition in vanadium dioxide and their hopping dynamics Article Swipe
Xiongfang Liu
,
Tong Yang
,
Jing Wu
,
Mengxia Sun
,
Mingyao Chen
,
Chi Sin Tang
,
Kun Han
,
Difan Zhou
,
Shengwei Zeng
,
Shuo Sun
,
Sensen Li
,
Ming Yang
,
Mark B. H. Breese
,
Chuanbing Cai
,
T. Venkatesan
,
Andrew T. S. Wee
,
Xinmao Yin
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2312.17419
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2312.17419
Researchers pursuing advanced photoelectric devices have discovered near room-temperature metal-insulator transitions (MIT) in non-volatile VO2. Despite theoretical investigations suggesting that polaron dynamics mediate the MIT, direct experimental evidence remains scarce. In this study, we present direct evidence of the polaron state in insulating VO2 through high-resolution spectroscopic ellipsometry measurements and first-principles calculations. We illustrate the complementary role of polaron dynamics in facilitating Peierls and Mott transitions, thereby contributing to the MIT processes. Furthermore, our observations and characterizations of conventional metallic and correlated plasmons in the respective phases of the VO2 film offer valuable insights into their electron structures. This investigation enhances comprehension of the MIT mechanism in correlated systems and underscores the roles of polarons, lattice distortions, and electron correlations in facilitating phase transition processes in strongly-correlated systems. Additionally, the detailed detection of small polarons and plasmons serves as inspiration for the development of new device functionalities.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2312.17419
- https://arxiv.org/pdf/2312.17419
- OA Status
- green
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4390489511
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4390489511Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2312.17419Digital Object Identifier
- Title
-
Small polarons mediated near-room-temperature metal-insulator transition in vanadium dioxide and their hopping dynamicsWork title
- Type
-
preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
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2023-12-29Full publication date if available
- Authors
-
Xiongfang Liu, Tong Yang, Jing Wu, Mengxia Sun, Mingyao Chen, Chi Sin Tang, Kun Han, Difan Zhou, Shengwei Zeng, Shuo Sun, Sensen Li, Ming Yang, Mark B. H. Breese, Chuanbing Cai, T. Venkatesan, Andrew T. S. Wee, Xinmao YinList of authors in order
- Landing page
-
https://arxiv.org/abs/2312.17419Publisher landing page
- PDF URL
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https://arxiv.org/pdf/2312.17419Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
-
https://arxiv.org/pdf/2312.17419Direct OA link when available
- Concepts
-
Polaron, Condensed matter physics, Photoelectric effect, Lattice (music), Metal–insulator transition, Electron, Plasmon, Vanadium, Materials science, Phase transition, Chemical physics, Metal, Physics, Optoelectronics, Quantum mechanics, Acoustics, MetallurgyTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
0Total citation count in OpenAlex
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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