Softened sp2-sp3 bonding network leads to strong anharmonicity and weak hydrodynamics in graphene+ Article Swipe
Linfeng Yu
,
Ailing Chen
,
Xiaoxia Wang
,
Huimin Wang
,
Zhenzhen Qin
,
Guangzhao Qin
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2204.07806
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2204.07806
Graphene+, a novel carbon monolayer with sp2-sp3 hybridization, is recently reported to exhibit graphene-like Dirac properties and unprecedented out-of-plane half-auxetic behavior [Yu et al, Cell Reports Physical Science, 3 100790 (2022)]. Herein, from comprehensively state-of-the-art first-principles studies, we report the exceptional lattice thermal transport properties of graphene+ driven by the unique sp2-sp3 crystal configuration. At room temperature, the thermal conductivity of graphene+ is calculated to be ~170 W/mK, which is much lower than that of graphene (~3170 W/mK) Despite the buckling structure, weak phonon scattering phase space is trapped in graphene+. Thus, the reduction in thermal conductivity magnitude stems from soft bonding due to the unique sp2-sp3 crystal configuration. Soft bonding suppresses the vibrations of acoustic phonons, which leads to strong anharmonicity and weak phonon hydrodynamics. Further, lower group velocity, relaxation time and smaller phonon mean free path emerge in graphene+, and the significantly decreased thermal conductivity is achieved. Our study provides fundamental physical insights into the thermal transport properties of graphene+, and it serves as an ideal model to study atomic bonding versus thermal transport properties due to weak scattering phase space.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2204.07806
- https://arxiv.org/pdf/2204.07806
- OA Status
- green
- Cited By
- 2
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4320169113
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4320169113Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2204.07806Digital Object Identifier
- Title
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Softened sp2-sp3 bonding network leads to strong anharmonicity and weak hydrodynamics in graphene+Work title
- Type
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preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-04-16Full publication date if available
- Authors
-
Linfeng Yu, Ailing Chen, Xiaoxia Wang, Huimin Wang, Zhenzhen Qin, Guangzhao QinList of authors in order
- Landing page
-
https://arxiv.org/abs/2204.07806Publisher landing page
- PDF URL
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https://arxiv.org/pdf/2204.07806Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
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https://arxiv.org/pdf/2204.07806Direct OA link when available
- Concepts
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Graphene, Anharmonicity, Phonon, Thermal conductivity, Condensed matter physics, Materials science, Scattering, Mean free path, Bilayer graphene, Nanotechnology, Physics, Optics, Composite materialTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
2Total citation count in OpenAlex
- Citations by year (recent)
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2025: 1, 2024: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.transport | 43, 158, 175 |
| abstract_inverted_index.velocity, | 129 |
| abstract_inverted_index.Graphene+, | 0 |
| abstract_inverted_index.calculated | 63 |
| abstract_inverted_index.graphene+, | 140, 161 |
| abstract_inverted_index.graphene+. | 90 |
| abstract_inverted_index.properties | 15, 44, 159, 176 |
| abstract_inverted_index.relaxation | 130 |
| abstract_inverted_index.scattering | 84, 180 |
| abstract_inverted_index.structure, | 81 |
| abstract_inverted_index.suppresses | 111 |
| abstract_inverted_index.vibrations | 113 |
| abstract_inverted_index.exceptional | 40 |
| abstract_inverted_index.fundamental | 152 |
| abstract_inverted_index.conductivity | 59, 96, 146 |
| abstract_inverted_index.half-auxetic | 19 |
| abstract_inverted_index.out-of-plane | 18 |
| abstract_inverted_index.temperature, | 56 |
| abstract_inverted_index.anharmonicity | 121 |
| abstract_inverted_index.graphene-like | 13 |
| abstract_inverted_index.significantly | 143 |
| abstract_inverted_index.unprecedented | 17 |
| abstract_inverted_index.configuration. | 53, 108 |
| abstract_inverted_index.hybridization, | 7 |
| abstract_inverted_index.hydrodynamics. | 125 |
| abstract_inverted_index.comprehensively | 33 |
| abstract_inverted_index.first-principles | 35 |
| abstract_inverted_index.state-of-the-art | 34 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 6 |
| citation_normalized_percentile |