Spatial Control of Substitutional Dopants in Hexagonal Monolayer WS2: The Effect of Edge Termination Article Swipe
Tianyi Zhang
,
Mingzu Liu
,
Kazunori Fujisawa
,
Michael Lucking
,
Kory Beach
,
Fu Zhang
,
Maruda Shanmugasundaram
,
Andrey Krayev
,
William Murray
,
Yu Lei
,
Zhuohang Yu
,
David Sánchez
,
Zhiwen Liu
,
Humberto Terrones
,
Ana Laura Elías
,
Mauricio Terrones
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/smll.202205800
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/smll.202205800
The ability to control the density and spatial distribution of substitutional dopants in semiconductors is crucial for achieving desired physicochemical properties. Substitutional doping with adjustable doping levels has been previously demonstrated in 2D transition metal dichalcogenides (TMDs); however, the spatial control of dopant distribution remains an open field. In this work, edge termination is demonstrated as an important characteristic of 2D TMD monocrystals that affects the distribution of substitutional dopants. Particularly, in chemical vapor deposition (CVD)‐grown monolayer WS 2 , it is found that a higher density of transition metal dopants is always incorporated in sulfur‐terminated domains when compared to tungsten‐terminated domains. Two representative examples demonstrate this spatial distribution control, including hexagonal iron‐ and vanadium‐doped WS 2 monolayers. Density functional theory (DFT) calculations are further performed, indicating that the edge‐dependent dopant distribution is due to a strong binding of tungsten atoms at tungsten‐zigzag edges, resulting in the formation of open sites at sulfur‐zigzag edges that enable preferential dopant incorporation. Based on these results, it is envisioned that edge termination in crystalline TMD monolayers can be utilized as a novel and effective knob for engineering the spatial distribution of substitutional dopants, leading to in‐plane hetero‐/multi‐junctions that display fascinating electronic, optoelectronic, and magnetic properties.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/smll.202205800
- OA Status
- green
- Cited By
- 25
- References
- 59
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4313424414
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4313424414Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/smll.202205800Digital Object Identifier
- Title
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Spatial Control of Substitutional Dopants in Hexagonal Monolayer WS2: The Effect of Edge TerminationWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-01-01Full publication date if available
- Authors
-
Tianyi Zhang, Mingzu Liu, Kazunori Fujisawa, Michael Lucking, Kory Beach, Fu Zhang, Maruda Shanmugasundaram, Andrey Krayev, William Murray, Yu Lei, Zhuohang Yu, David Sánchez, Zhiwen Liu, Humberto Terrones, Ana Laura Elías, Mauricio TerronesList of authors in order
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https://doi.org/10.1002/smll.202205800Publisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/1923824Direct OA link when available
- Concepts
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Dopant, Monolayer, Enhanced Data Rates for GSM Evolution, Hexagonal crystal system, Materials science, Condensed matter physics, Crystallography, Nanotechnology, Chemical physics, Optoelectronics, Doping, Physics, Computer science, Chemistry, TelecommunicationsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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25Total citation count in OpenAlex
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2025: 5, 2024: 13, 2023: 7Per-year citation counts (last 5 years)
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59Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| corresponding_author_ids | https://openalex.org/A5055072817, https://openalex.org/A5030207185, https://openalex.org/A5069865883 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 16 |
| corresponding_institution_ids | https://openalex.org/I123946342, https://openalex.org/I130769515, https://openalex.org/I165799507 |
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| sustainable_development_goals[0].display_name | Clean water and sanitation |
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