Stochasticity in materials structure, properties, and processing—A review Article Swipe
R. Hull
,
Pawel Keblinski
,
Dan Lewis
,
Antoinette M. Maniatty
,
Vincent Meunier
,
Assad A. Oberai
,
Catalin R. Picu
,
Johnson Samuel
,
Mark S. Shephard
,
M. Tomozawa
,
Deepak Vashishth
,
Shengbai Zhang
·
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.1063/1.4998144
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.1063/1.4998144
We review the concept of stochasticity—i.e., unpredictable or uncontrolled fluctuations in structure, chemistry, or kinetic processes—in materials. We first define six broad classes of stochasticity: equilibrium (thermodynamic) fluctuations; structural/compositional fluctuations; kinetic fluctuations; frustration and degeneracy; imprecision in measurements; and stochasticity in modeling and simulation. In this review, we focus on the first four classes that are inherent to materials phenomena. We next develop a mathematical framework for describing materials stochasticity and then show how it can be broadly applied to these four materials-related stochastic classes. In subsequent sections, we describe structural and compositional fluctuations at small length scales that modify material properties and behavior at larger length scales; systems with engineered fluctuations, concentrating primarily on composite materials; systems in which stochasticity is developed through nucleation and kinetic phenomena; and configurations in which constraints in a given system prevent it from attaining its ground state and cause it to attain several, equally likely (degenerate) states. We next describe how stochasticity in these processes results in variations in physical properties and how these variations are then accentuated by—or amplify—stochasticity in processing and manufacturing procedures. In summary, the origins of materials stochasticity, the degree to which it can be predicted and/or controlled, and the possibility of using stochastic descriptions of materials structure, properties, and processing as a new degree of freedom in materials design are described.
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- Type
- article
- Language
- en
- Landing Page
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- OA Status
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- Cited By
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All OpenAlex metadata
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https://doi.org/10.1063/1.4998144Digital Object Identifier
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Stochasticity in materials structure, properties, and processing—A reviewWork title
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articleOpenAlex work type
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enPrimary language
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2018Year of publication
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2018-03-01Full publication date if available
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R. Hull, Pawel Keblinski, Dan Lewis, Antoinette M. Maniatty, Vincent Meunier, Assad A. Oberai, Catalin R. Picu, Johnson Samuel, Mark S. Shephard, M. Tomozawa, Deepak Vashishth, Shengbai ZhangList of authors in order
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.ncbi.nlm.nih.gov/pmc/articles/6214486Direct OA link when available
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2025: 7, 2024: 1, 2023: 1, 2022: 5, 2021: 4Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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