Strong Neel Ordering and Luminescence Correlation in a Two‐Dimensional Antiferromagnet Article Swipe
Yongheng Zhou
,
Kaiyue He
,
Huamin Hu
,
Gangfeng Ouyang
,
Chao Zhu
,
Wei Wang
,
Sichen Qin
,
Ye Tao
,
Runfeng Chen
,
Le Zhang
,
Run Shi
,
Chun Cheng
,
Han Wang
,
Yanjun Liu
,
Zheng Liu
,
Taihong Wang
,
Wei Huang
,
Lin Wang
,
Xiaolong Chen
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1002/lpor.202100431
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1002/lpor.202100431
Magneto‐optical effect has been widely used in light modulation, optical sensing, and information storage. Recently discovered 2D van der Waals layered magnets are considered as promising platforms for investigating novel magneto‐optical phenomena and devices, due to the long‐range magnetic ordering down to atomically thin thickness, rich species, and tunable properties. However, majority 2D antiferromagnets suffer from low luminescence efficiency which hinders their magneto‐optical investigations and applications. This work uncovers strong light‐magnetic ordering interactions in 2D antiferromagnetic MnPS 3 using a newly‐emerged near‐infrared photoluminescence (PL) mode far below its intrinsic bandgap. This ingap PL mode shows strong correlation with the Neel ordering and persists down to monolayer thickness. Combining the density‐functional theory (DFT), scanning transmission electron microscopy (STEM), and X‐ray photoelectron spectroscopy (XPS), this work illustrates the origin of the PL mode and its correlation with Neel ordering, which can be attributed to the oxygen ion‐mediated states. Moreover, the PL strength can be further tuned and enhanced using ultraviolet‐ozone (UVO) treatment. The studies offer an effective approach to investigate light‐magnetic ordering interactions in 2D antiferromagnetic semiconductors.
Related Topics
Concepts
Antiferromagnetism
Materials science
Ferromagnetism
Néel temperature
Photoluminescence
Condensed matter physics
van der Waals force
X-ray photoelectron spectroscopy
Density functional theory
Band gap
Luminescence
Monolayer
Optoelectronics
Nanotechnology
Chemistry
Physics
Magnetic field
Nuclear magnetic resonance
Magnetization
Computational chemistry
Molecule
Organic chemistry
Quantum mechanics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/lpor.202100431
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/lpor.202100431
- OA Status
- bronze
- Cited By
- 11
- References
- 61
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4280558802
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4280558802Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/lpor.202100431Digital Object Identifier
- Title
-
Strong Neel Ordering and Luminescence Correlation in a Two‐Dimensional AntiferromagnetWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-06-19Full publication date if available
- Authors
-
Yongheng Zhou, Kaiyue He, Huamin Hu, Gangfeng Ouyang, Chao Zhu, Wei Wang, Sichen Qin, Ye Tao, Runfeng Chen, Le Zhang, Run Shi, Chun Cheng, Han Wang, Yanjun Liu, Zheng Liu, Taihong Wang, Wei Huang, Lin Wang, Xiaolong ChenList of authors in order
- Landing page
-
https://doi.org/10.1002/lpor.202100431Publisher landing page
- PDF URL
-
https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/lpor.202100431Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
bronzeOpen access status per OpenAlex
- OA URL
-
https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/lpor.202100431Direct OA link when available
- Concepts
-
Antiferromagnetism, Materials science, Ferromagnetism, Néel temperature, Photoluminescence, Condensed matter physics, van der Waals force, X-ray photoelectron spectroscopy, Density functional theory, Band gap, Luminescence, Monolayer, Optoelectronics, Nanotechnology, Chemistry, Physics, Magnetic field, Nuclear magnetic resonance, Magnetization, Computational chemistry, Molecule, Organic chemistry, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
11Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 4, 2024: 4, 2023: 2, 2022: 1Per-year citation counts (last 5 years)
- References (count)
-
61Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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