Strongly Anisotropic Charge Dynamics in La3Ni2O7 with Coherent-to-Incoherent Crossover of Interlayer Charge Dynamics Article Swipe
Bo Su
,
Chaoxin Huang
,
Jianzhou Zhao
,
Mengwu Huo
,
Jianlin Luo
,
Meng Wang
,
Zhiguo Chen
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2411.10786
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2411.10786
We report an optical spectroscopy study of the charge-dynamics anisotropy in the La3Ni2O7 single crystals with the electric field of the incident light parallel to the crystalline c-axis and ab-plane respectively. The evolution of the low-energy part of its c-axis optical conductivity spectra (σ1c(ω)) from a Drude component to a finite-energy peak, together with the change in the c-axis electron mean-free-path which is distinctly longer than the c-axis lattice constant at 10 K but is shorter than the c-axis lattice constant at 300 K, demonstrates a crossover from coherent to incoherent interlayer charge dynamics in La3Ni2O7, which is associated with the variation from weak to strong dissipation within its ab-plane. In contrast, the Drude component robust in its σ1ab(ω) and the long ab-plane electron mean-free-path greater than the a-axis and b-axis unit-cell lengths manifest the persistence of coherent in-plane charge dynamics from 10 to 300 K. Thus, the charge dynamics in La3Ni2O7 shows a remarkable anisotropy at high temperatures. At low temperatures, the large values of the ratio between the ab-plane and c-axis Drude weights and the ratio σ1ab(ω -> 0)/σ1c(ω -> 0) indicate a strong anisotropy of the low-temperature charge dynamics in La3Ni2O7.
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- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2411.10786
- https://arxiv.org/pdf/2411.10786
- OA Status
- green
- Related Works
- 10
- OpenAlex ID
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https://openalex.org/W4404570193Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2411.10786Digital Object Identifier
- Title
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Strongly Anisotropic Charge Dynamics in La3Ni2O7 with Coherent-to-Incoherent Crossover of Interlayer Charge DynamicsWork title
- Type
-
preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-11-16Full publication date if available
- Authors
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Bo Su, Chaoxin Huang, Jianzhou Zhao, Mengwu Huo, Jianlin Luo, Meng Wang, Zhiguo ChenList of authors in order
- Landing page
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https://arxiv.org/abs/2411.10786Publisher landing page
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https://arxiv.org/pdf/2411.10786Direct link to full text PDF
- Open access
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://arxiv.org/pdf/2411.10786Direct OA link when available
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Charge (physics), Dynamics (music), Crossover, Anisotropy, Physics, Condensed matter physics, Statistical physics, Molecular dynamics, Chemical physics, Quantum mechanics, Computer science, Acoustics, Artificial intelligenceTop concepts (fields/topics) attached by OpenAlex
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| abstract_inverted_index.remarkable | 154 |
| abstract_inverted_index.crystalline | 26 |
| abstract_inverted_index.dissipation | 106 |
| abstract_inverted_index.persistence | 135 |
| abstract_inverted_index.conductivity | 41 |
| abstract_inverted_index.demonstrates | 84 |
| abstract_inverted_index.spectroscopy | 4 |
| abstract_inverted_index.finite-energy | 50 |
| abstract_inverted_index.respectively. | 30 |
| abstract_inverted_index.temperatures, | 161 |
| abstract_inverted_index.temperatures. | 158 |
| abstract_inverted_index.mean-free-path | 60, 124 |
| abstract_inverted_index.charge-dynamics | 8 |
| abstract_inverted_index.low-temperature | 189 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 7 |
| citation_normalized_percentile |