Sulfhydryl‐functionalized COF‐based electrolyte strengthens chemical affinity toward polysulfides in quasi‐solid‐state Li‐S batteries Article Swipe
Linnan Bi
,
Jie Xiao
,
Yaochen Song
,
Tianrui Sun
,
Mingkai Luo
,
Yi Wang
,
Peng Dong
,
Yingjie Zhang
,
Yao Yao
,
Jiaxuan Liao
,
Sizhe Wang
,
Shulei Chou
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/cey2.544
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/cey2.544
For lithium‐sulfur batteries (Li‐S batteries), a high‐content electrolyte typically can exacerbate the shuttle effect, while a lean electrolyte may lead to decreased Li‐ion conductivity and reduced catalytic conversion efficiency, so achieving an appropriate electrolyte‐to‐sulfur ratio (E/S ratio) is essential for improving the battery cycling efficiency. A quasi‐solid electrolyte (COF‐SH@PVDF‐HFP) with strong adsorption and high catalytic conversion was constructed for in situ covalent organic framework (COF) growth on highly polarized polyvinylidene fluoride‐hexafluoropropylene (PVDF‐HFP) fibers. COF‐SH@PVDF‐HFP enables efficient Li‐ion conductivity with low‐content liquid electrolyte and effectively suppresses the shuttle effect. The results based on in situ Fourier‐transform infrared, in situ Raman, UV–Vis, X‐ray photoelectron, and density functional theory calculations confirmed the high catalytic conversion of COF‐SH layer containing sulfhydryl and imine groups for the lithium polysulfides. Lithium plating/stripping tests based on Li/COF‐SH@PVDF‐HFP/Li show excellent lithium compatibility (5 mAh cm −2 for 1400 h). The assembled Li‐S battery exhibits excellent rate (2 C 688.7 mAh g −1 ) and cycle performance (at 2 C of 568.8 mAh g −1 with a capacity retention of 77.3% after 800 cycles). This is the first report to improve the cycling stability of quasi‐solid‐state Li‐S batteries by reducing both the E/S ratio and the designing strategy of sulfhydryl‐functionalized COF for quasi‐solid electrolytes. This process opens up the possibility of the high performance of solid‐state Li‐S batteries.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/cey2.544
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cey2.544
- OA Status
- gold
- Cited By
- 34
- References
- 63
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4394881145
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- OpenAlex ID
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https://openalex.org/W4394881145Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/cey2.544Digital Object Identifier
- Title
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Sulfhydryl‐functionalized COF‐based electrolyte strengthens chemical affinity toward polysulfides in quasi‐solid‐state Li‐S batteriesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-04-17Full publication date if available
- Authors
-
Linnan Bi, Jie Xiao, Yaochen Song, Tianrui Sun, Mingkai Luo, Yi Wang, Peng Dong, Yingjie Zhang, Yao Yao, Jiaxuan Liao, Sizhe Wang, Shulei ChouList of authors in order
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https://doi.org/10.1002/cey2.544Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cey2.544Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cey2.544Direct OA link when available
- Concepts
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Electrolyte, Chemical engineering, Conductivity, Polyvinylidene fluoride, Catalysis, Lithium–sulfur battery, Raman spectroscopy, Materials science, Chemistry, Inorganic chemistry, Electrode, Membrane, Organic chemistry, Physical chemistry, Physics, Optics, Engineering, BiochemistryTop concepts (fields/topics) attached by OpenAlex
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34Total citation count in OpenAlex
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2025: 31, 2024: 3Per-year citation counts (last 5 years)
- References (count)
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63Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.show | 131 |
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| abstract_inverted_index.−1 | 154, 166 |
| abstract_inverted_index.−2 | 138 |
| abstract_inverted_index.(COF) | 65 |
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| abstract_inverted_index.688.7 | 151 |
| abstract_inverted_index.77.3% | 172 |
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| abstract_inverted_index.ratio | 35, 195 |
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| abstract_inverted_index.Li‐S | 144, 188, 218 |
| abstract_inverted_index.Raman, | 99 |
| abstract_inverted_index.groups | 120 |
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| abstract_inverted_index.highly | 68 |
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| abstract_inverted_index.X‐ray | 101 |
| abstract_inverted_index.battery | 43, 145 |
| abstract_inverted_index.cycling | 44, 184 |
| abstract_inverted_index.density | 104 |
| abstract_inverted_index.effect, | 14 |
| abstract_inverted_index.effect. | 88 |
| abstract_inverted_index.enables | 75 |
| abstract_inverted_index.fibers. | 73 |
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| abstract_inverted_index.covalent | 62 |
| abstract_inverted_index.cycles). | 175 |
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| abstract_inverted_index.reducing | 191 |
| abstract_inverted_index.strategy | 199 |
| abstract_inverted_index.UV–Vis, | 100 |
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| abstract_inverted_index.possibility | 211 |
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| abstract_inverted_index.compatibility | 134 |
| abstract_inverted_index.electrolytes. | 205 |
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| abstract_inverted_index.polyvinylidene | 70 |
| abstract_inverted_index.lithium‐sulfur | 2 |
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| abstract_inverted_index.Fourier‐transform | 95 |
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| abstract_inverted_index.fluoride‐hexafluoropropylene | 71 |
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| cited_by_percentile_year.min | 96 |
| corresponding_author_ids | https://openalex.org/A5020275874, https://openalex.org/A5100389416, https://openalex.org/A5039658876, https://openalex.org/A5056158205 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 12 |
| corresponding_institution_ids | https://openalex.org/I10660446, https://openalex.org/I146620803, https://openalex.org/I150229711, https://openalex.org/I4210123686, https://openalex.org/I51622183 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
| sustainable_development_goals[0].score | 0.6200000047683716 |
| sustainable_development_goals[0].display_name | Affordable and clean energy |
| citation_normalized_percentile.value | 0.98615718 |
| citation_normalized_percentile.is_in_top_1_percent | True |
| citation_normalized_percentile.is_in_top_10_percent | True |