Sulfur‐Rich Norbornadiene‐Derived Infrared Transparent Polymers by Inverse Vulcanization Article Swipe
Yishun Wuliu
,
Weiliang Dong
,
Guohua Huang
,
Hui Xie
,
Pingping Yao
,
Jiji Tan
,
Kexin Mu
,
Zhi-Li Zhang
,
Yinan Chen
,
Mingliang Wang
,
Lei Tian
,
Caizhen Zhu
,
Jian Xu
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202419446
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202419446
Infrared (IR) transparent polymer materials prepared by inverse vulcanization, as a promising candidate to replace inorganic materials, are new materials for constructing key devices in IR optics. However, it is difficult to achieve a balance between infrared optical and thermal properties in polymers due to the intrinsic infrared absorption of organic materials. Herein, our strategy is to construct a high boiling point symmetrical molecular norbornadiene derivative cross‐linking agent (DMMD) which can be inverse vulcanized with molten sulfur, and obtain Poly (S‐r‐DMMD) with different sulfur content by controlling the feed ratio of sulfur. With the rigid core and low IR activity in DMMD, the prepared polymers exhibit tunable thermal properties ( T g : 98.3–119.8 °C) and high IR transmittance (medium‐wave infrared region (MWIR): 42.9–52.6 %; long‐wave infrared region (LWIR): 1.5–5.29 %). In addition, Poly (S‐r‐DMMD) can be used to prepare large‐size free‐standing Fresnel lenses for IR imaging by simple hot‐pressing, which provides flexibility in the design and production of IR fine lenses. This study provides a novel strategy for balancing the thermal and optical properties of IR transparent polymer materials, while providing relevant references for balancing the IR optical and thermal properties of polymer materials.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/anie.202419446
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202419446
- OA Status
- bronze
- Cited By
- 7
- References
- 51
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4403915720
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- OpenAlex ID
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https://openalex.org/W4403915720Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/anie.202419446Digital Object Identifier
- Title
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Sulfur‐Rich Norbornadiene‐Derived Infrared Transparent Polymers by Inverse VulcanizationWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-10-29Full publication date if available
- Authors
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Yishun Wuliu, Weiliang Dong, Guohua Huang, Hui Xie, Pingping Yao, Jiji Tan, Kexin Mu, Zhi-Li Zhang, Yinan Chen, Mingliang Wang, Lei Tian, Caizhen Zhu, Jian XuList of authors in order
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https://doi.org/10.1002/anie.202419446Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202419446Direct link to full text PDF
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202419446Direct OA link when available
- Concepts
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Infrared, Materials science, Vulcanization, Polymer, Norbornadiene, Optics, Composite material, Organic chemistry, Chemistry, Natural rubber, Physics, CatalysisTop concepts (fields/topics) attached by OpenAlex
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7Total citation count in OpenAlex
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2025: 7Per-year citation counts (last 5 years)
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51Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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