Suppression of Cation Intermixing Highly Boosts the Performance of Core–Shell Lanthanide Upconversion Nanoparticles Article Swipe
Fuhua Huang
,
Niusha Bagheri
,
Li Wang
,
Hans Ågren
,
Jinglai Zhang
,
Rui Pu
,
Qiuqiang Zhan
,
Yuhan Jing
,
Wen Xu
,
Jerker Widengren
,
Haichun Liu
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/jacs.3c03019
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/jacs.3c03019
Lanthanide upconversion nanoparticles (UCNPs) have been extensively explored as biomarkers, energy transducers, and information carriers in wide-ranging applications in areas from healthcare and energy to information technology. In promoting the brightness and enriching the functionalities of UCNPs, core-shell structural engineering has been well-established as an important approach. Despite its importance, a strong limiting issue has been identified, namely, cation intermixing in the interfacial region of the synthesized core-shell nanoparticles. Currently, there still exists confusion regarding this destructive phenomenon and there is a lack of facile means to reach a delicate control of it. By means of a new set of experiments, we identify and provide in this work a comprehensive picture for the major physical mechanism of cation intermixing occurring in synthesis of core-shell UCNPs, i.e., partial or substantial core nanoparticle dissolution followed by epitaxial growth of the outer layer and ripening of the entire particle. Based on this picture, we provide an easy but effective approach to tackle this issue that enables us to produce UCNPs with highly boosted optical properties.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/jacs.3c03019
- OA Status
- hybrid
- Cited By
- 38
- References
- 47
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4385638490
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4385638490Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/jacs.3c03019Digital Object Identifier
- Title
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Suppression of Cation Intermixing Highly Boosts the Performance of Core–Shell Lanthanide Upconversion NanoparticlesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
-
2023-08-07Full publication date if available
- Authors
-
Fuhua Huang, Niusha Bagheri, Li Wang, Hans Ågren, Jinglai Zhang, Rui Pu, Qiuqiang Zhan, Yuhan Jing, Wen Xu, Jerker Widengren, Haichun LiuList of authors in order
- Landing page
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https://doi.org/10.1021/jacs.3c03019Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1021/jacs.3c03019Direct OA link when available
- Concepts
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Nanoparticle, Chemistry, Lanthanide, Nanotechnology, Photon upconversion, Core (optical fiber), Limiting, Particle (ecology), Ion, Materials science, Computer science, Telecommunications, Oceanography, Geology, Engineering, Organic chemistry, Mechanical engineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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38Total citation count in OpenAlex
- Citations by year (recent)
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2025: 22, 2024: 16Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| corresponding_institution_ids | https://openalex.org/I173899330, https://openalex.org/I86987016 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
| sustainable_development_goals[0].score | 0.5299999713897705 |
| sustainable_development_goals[0].display_name | Affordable and clean energy |
| citation_normalized_percentile.value | 0.95722816 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |