Suppression of ferromagnetism in van der Waals insulator due to pressure-induced layer stacking variation Article Swipe
Martin Míšek
,
U. Dutta
,
Pavel Král
,
David Hovancik
,
J. Kaštil
,
K. Pokhrel
,
Sugata Ray
,
J. Valenta
,
J. Prchal
,
J. Kamarád
,
Fedir Borodavka
,
Václav Eigner
,
Michal Dušek
,
V. Holý
,
K. Carva
,
S. Kamba
,
V. Sechovský
,
Jiří Pospíšil
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2501.13446
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2501.13446
External pressure suppresses the ferromagnetism of localized Cr 3d electron moments in the van der Waals insulator CrBr3, which cannot be explained without considering a dramatic pressure-induced crystal or electronic structure change. We addressed this issue by conducting a parallel experimental investigation of single crystals magnetic and structural properties using magnetization, X-ray diffraction, and Raman spectroscopy measurements. Ab initio DFT calculations of electronic structure and atomistic simulations of finite-temperature magnetism supported the analysis and interpretation of experimental results. The magnetization measurements at high pressures provided the first direct experimental evidence of the pressure-induced suppression of ferromagnetism. We observed a gradual decrease of the bulk magnetic moment and Curie temperature with increasing pressure, which accelerates at pressures above 3 GPa, leading to loss of ferromagnetism at 6.5 GPa. By increasing pressure, the ambient pressure phase gradually breaks down and is accompanied by the generation of layer stacking that favor the antiferromagnetic coupling of Cr moments. As a result, the appearing antiparallel pairs of moments disturb the ferromagnetic structure and reduce the bulk magnetic moment and Curie temperature. This scenario, which is well corroborated by the results of our theoretical calculations, suggests an antiferromagnetic phase emerging with increasing pressure beyond the critical value when the new single trigonal P-3m1 phase becomes stable, characterized by the "antiferromagnetic" A-A layer stacking, becomes stable. The weak coupling between adjacent magnetic layers in van der Waals materials allows variations in layering due to sufficient external forces. We hope our comprehensive study's results can help other researchers resolve frequently appearing issues of similar origin in this class of materials.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2501.13446
- https://arxiv.org/pdf/2501.13446
- OA Status
- green
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4406786117
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4406786117Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2501.13446Digital Object Identifier
- Title
-
Suppression of ferromagnetism in van der Waals insulator due to pressure-induced layer stacking variationWork title
- Type
-
preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-01-23Full publication date if available
- Authors
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Martin Míšek, U. Dutta, Pavel Král, David Hovancik, J. Kaštil, K. Pokhrel, Sugata Ray, J. Valenta, J. Prchal, J. Kamarád, Fedir Borodavka, Václav Eigner, Michal Dušek, V. Holý, K. Carva, S. Kamba, V. Sechovský, Jiří PospíšilList of authors in order
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https://arxiv.org/abs/2501.13446Publisher landing page
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https://arxiv.org/pdf/2501.13446Direct link to full text PDF
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://arxiv.org/pdf/2501.13446Direct OA link when available
- Concepts
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Stacking, Condensed matter physics, Ferromagnetism, van der Waals force, Materials science, Insulator (electricity), Variation (astronomy), Layer (electronics), Physics, Nanotechnology, Nuclear magnetic resonance, Composite material, Quantum mechanics, Astrophysics, MoleculeTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| publication_date | 2025-01-23 |
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