Synchronously Stabilizing the Interphase of Cathode and Anode Enabling Lithium Metal Batteries via Multiple Electrolyte Additives Article Swipe
Yi Wan
,
Wenjiang Bai
,
Shun Wu
,
Che Sun
,
Shuaishuai Chen
,
Yinping Qin
,
Muqin Wang
,
Zhenlian Chen
,
Mingkui Wang
,
Deyu Wang
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/batteries10100338
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/batteries10100338
As the most promising high energy density technology, lithium metal batteries are associated with serious interfacial challenges because the electrolytes employed are unable to meet the requirements of both electrodes simultaneously, namely, the systems that work for Li metal are highly likely to be unsuitable for the cathode, and vice versa. In this study, we investigate the synergistic effects of lithium bis (oxalate) borate (LiBOB), fluoroethylene carbonate (FEC) and adiponitrile (ADN) to develop a formula that is compatible with both elements in the battery. The solid–electrolyte interphase (SEI) multi-layer generated from LiBOB and FEC successfully protects the electrolyte from the lithium and suppresses the decomposition of ADN on lithium, identified by the tiny amounts of isonitriles on the surface of the anode. Simultaneously, most of the ADN molecules remain and protect the cathode particles via the absorption layer of the nitrile groups, in the same way that this process works in commercial lithium-ion batteries. Benefiting from the stable interfacial films formed synchronously on the anode and cathode, the Li/LiNi0.8Co0.1Mn0.1O2 cells with an area capacity of ~3 mAh cm−2 operate stably beyond 250 cycles and target the accumulated capacity to levels as high as ~653.4 mAh cm−2. Our approach demonstrates that electrolyte engineering with known additives is a practical strategy for addressing the challenges of lithium batteries.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/batteries10100338
- OA Status
- gold
- References
- 23
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
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https://openalex.org/W4402759460Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/batteries10100338Digital Object Identifier
- Title
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Synchronously Stabilizing the Interphase of Cathode and Anode Enabling Lithium Metal Batteries via Multiple Electrolyte AdditivesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-09-24Full publication date if available
- Authors
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Yi Wan, Wenjiang Bai, Shun Wu, Che Sun, Shuaishuai Chen, Yinping Qin, Muqin Wang, Zhenlian Chen, Mingkui Wang, Deyu WangList of authors in order
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https://doi.org/10.3390/batteries10100338Publisher landing page
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
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https://doi.org/10.3390/batteries10100338Direct OA link when available
- Concepts
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Anode, Electrolyte, Cathode, Interphase, Lithium metal, Materials science, Lithium (medication), Metal, Chemical engineering, Inorganic chemistry, Electrode, Chemistry, Metallurgy, Physical chemistry, Biology, Medicine, Engineering, Endocrinology, GeneticsTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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