Synergistic Effect of Solvent and Component Engineering for High‐Efficiency Carbon‐Based Perovskite Solar Cells Article Swipe

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Nannan Wang , Jiating Wang , Xinrui Gao , Yingjia Zhuansun , Decai Zhu , Qingbo Wei , Shengzhong Liu ·

YOU? · · 2025 · Open Access · · DOI: https://doi.org/10.1002/smtd.202402039

It is highly desired to get rid of the high‐temperature annealing process in manufacturing perovskite solar cells (PSCs) to reduce production costs. Herein, perovskite films are designed by rapidly evaporating of a mixture solvent consisting of methylamine ethanol solution (MA‐EtOH sol) and acetonitrile (ACN) (MA‐EtOH‐ACN) by dopping different amounts of formamidinium iodide (FAI) into the CH 3 NH 2 PbI 3 (MAPbI 3 ) precursor solution; as a result, the high‐temperature annealing step is effectively eliminated while the perovskite solar cell efficiency remains unchanged. The in situ UV–vis absorption for monitoring the perovskite crystallization process shows that FAI retards the crystallization rate, leading to a dense and smooth film. It is also found that the synergistic effect of solvent and composition engineering reduces defect density, boosts absorption strength, and enhances film stability. Consequently, high‐performance ITO/SnO 2 /FA 0.05 MA 0.95 PbI 3 /carbon device is obtained with efficiency as high as 18.74%, with an excellent short circuit current of 25.04 mA cm −2 , an open circuit voltage of 1.16 V, and a fill factor of 64.53%. The carbon‐based perovskite solar cells also exhibit outstanding stability. This strategy offers a reference to producing efficient and stable perovskite cells by the straightforward ink method.

Related Topics

Crystallization

Materials Science

Perovskite (Structure)

Chemical Engineering

Solvent

Potassium Iodide

Perovskite Solar Cell

Electrical Engineering

Engineering

Concepts

Crystallization Annealing (glass) Materials science Perovskite (structure) Chemical engineering Solvent Iodide Formamidinium Methylamine Energy conversion efficiency Acetonitrile Perovskite solar cell Solar cell Open-circuit voltage Photovoltaic system Chemistry Inorganic chemistry Organic chemistry Optoelectronics Composite material Voltage Electrical engineering Engineering

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Type: article
Language: en
Landing Page: https://doi.org/10.1002/smtd.202402039
PDF: https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/smtd.202402039
OA Status: bronze
Cited By: 1
References: 55
Related Works: 10
OpenAlex ID: https://openalex.org/W4408245476

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DOI: https://doi.org/10.1002/smtd.202402039

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Title: Synergistic Effect of Solvent and Component Engineering for High‐Efficiency Carbon‐Based Perovskite Solar Cells

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Type: article

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Language: en

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Publication year: 2025

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Publication date: 2025-03-04

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Authors: Nannan Wang, Jiating Wang, Xinrui Gao, Yingjia Zhuansun, Decai Zhu, Qingbo Wei, Shengzhong Liu

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Landing page: https://doi.org/10.1002/smtd.202402039

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Concepts: Crystallization, Annealing (glass), Materials science, Perovskite (structure), Chemical engineering, Solvent, Iodide, Formamidinium, Methylamine, Energy conversion efficiency, Acetonitrile, Perovskite solar cell, Solar cell, Open-circuit voltage, Photovoltaic system, Chemistry, Inorganic chemistry, Organic chemistry, Optoelectronics, Composite material, Voltage, Electrical engineering, Engineering

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Cited by: 1

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