Synthesis and Luminescence of Oligomers Containing Multiple Styrene Chromophores Regioselectively Separated by 2,2‐Propylidene and 1,2‐Isobutylidene Bridges Article Swipe
Qianqian Hu
,
Zhengfei Zhuang
,
Yun‐Shiuan Leung
,
Kejiang Liang
,
Meihua Yang
,
Hua Lü
,
Zhichang Liu
,
Guoqiao Lai
,
Tien‐Yau Luh
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/marc.202401075
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/marc.202401075
Oligomers incorporating styrene chromophores, linked by 1,2‐isobutylidene and 2,2‐propylidene spacers in various proportions, are synthesized through the NiCl 2 (PPh 3 ) 2 ‐catalyzed olefination‐oligomerization of benzene‐bisdithioacetal under diverse conditions using excess MeMgI and ZnI 2 . The method provides a convenient pathway for selectively synthesizing oligomers with distinct ratios of one‐carbon and two‐carbon linkers, strategically employed to spatially separate adjacent vinylarene chromophores. The emission profiles for these oligomers span from 380 to 450 nm, in addition to the intrinsic emission of styrene ≈315 nm. The intensity of the blue light emission varies depending on the ratio of the aliphatic linkers, attributed to through‐space intrachain ground‐state interactions among the styrene chromophores. Consequently, emission properties can be finely tuned; π‐conjugated chromophores enriched with 2,2‐propylidene linkers display higher luminescence intensity with discernible vibronic structure compared to those with higher percentages of 1,2‐isobutylidene spacers. This difference underscores the folding behaviors of the oligomers, where even slight structural variations in the oligomer structure can markedly influence their 3D conformation. Importantly, these experimental findings are corroborated by molecular dynamic simulations.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/marc.202401075
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/marc.202401075
- OA Status
- bronze
- References
- 50
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4408244899
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https://openalex.org/W4408244899Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/marc.202401075Digital Object Identifier
- Title
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Synthesis and Luminescence of Oligomers Containing Multiple Styrene Chromophores Regioselectively Separated by 2,2‐Propylidene and 1,2‐Isobutylidene BridgesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-03-06Full publication date if available
- Authors
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Qianqian Hu, Zhengfei Zhuang, Yun‐Shiuan Leung, Kejiang Liang, Meihua Yang, Hua Lü, Zhichang Liu, Guoqiao Lai, Tien‐Yau LuhList of authors in order
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https://doi.org/10.1002/marc.202401075Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/marc.202401075Direct link to full text PDF
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/marc.202401075Direct OA link when available
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Chromophore, Luminescence, Oligomer, Styrene, Conjugated system, Photochemistry, Chemistry, Benzene, Materials science, Polymer chemistry, Copolymer, Polymer, Organic chemistry, OptoelectronicsTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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