Synthesis of Two Structurally Different MgO Films Containing Dioxygen Species: Dioxygen Embedded at Grain Boundaries, and as Components of a Superfilled Rock Salt Structure Article Swipe
D. Fischer
,
Dejan Zagorac
,
Kathrin Küster
,
J. Christian Schön
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/coatings14121563
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/coatings14121563
Magnesium oxide films prepared as monolayer, amorphous, and epitaxial films have different properties such as semiconducting, ferromagnetic, and dielectric behavior, respectively. Understanding the variation in these properties requires detailed information about the atomic structure of the different MgO films. In the present study, one important synthesis method, ballistic deposition, is studied, and the influence of the deposition temperature on the resulting atomic structure of the films is analyzed in detail, employing XRD, SEM, EDX, XPS, and Raman scattering. At −190 °C, compact, light-yellow films are obtained, which consist of small crystallites adopting the rock salt structure with an excess of oxygen at the grain boundaries. However, at 25 °C, nearly stoichiometric, white, columnar films exhibiting a superfilled rock salt structure are grown. In the first case, dioxygen species are formed by connecting the oxygen shells of adjacent small crystalline grains, and in the second case such species appear due to the partial occupation of tetrahedral sites in the rock salt structure. These observations should open new prospects of fine-tuning the properties of MgO films and enhance the performance of devices employing such films.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/coatings14121563
- OA Status
- gold
- Cited By
- 6
- References
- 90
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
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https://openalex.org/W4405365945Canonical identifier for this work in OpenAlex
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https://doi.org/10.3390/coatings14121563Digital Object Identifier
- Title
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Synthesis of Two Structurally Different MgO Films Containing Dioxygen Species: Dioxygen Embedded at Grain Boundaries, and as Components of a Superfilled Rock Salt StructureWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
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2024Year of publication
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2024-12-13Full publication date if available
- Authors
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D. Fischer, Dejan Zagorac, Kathrin Küster, J. Christian SchönList of authors in order
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https://doi.org/10.3390/coatings14121563Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.3390/coatings14121563Direct OA link when available
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Salt (chemistry), Grain boundary, Oxygen, Materials science, Chemistry, Mineralogy, Chemical engineering, Crystallography, Microstructure, Organic chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
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6Total citation count in OpenAlex
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2025: 6Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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