Tailorable Multi‐Modular Pore‐Space‐Partitioned Vanadium Metal‐Organic Frameworks for Gas Separation Article Swipe
Wei Wang
,
Yichong Chen
,
Pingyun Feng
,
Xianhui Bu
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202403834
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202403834
Currently, few porous vanadium metal‐organic frameworks (V‐MOFs) are known and even fewer are obtainable as single crystals, resulting in limited information on their structures and properties. Here this work demonstrates remarkable promise of V‐MOFs by presenting an extensible family of V‐MOFs with tailorable pore geometry and properties. The synthesis leverages inter‐modular synergy on a tri‐modular pore‐partitioned platform. New V‐MOFs show a broad range of structural features and sorption properties suitable for gas storage and separation applications for C 2 H 2 /CO 2 , C 2 H 6 /C 2 H 4 , and C 3 H 8 /C 3 H 6 . The c / a ratio of the hexagonal cell, a measure of pore shape, is tunable from 0.612 to 1.258. Other tunable properties include pore size from 5.0 to 10.9 Å and surface area from 820 to 2964 m 2 g −1 . With C 2 H 2 /CO 2 selectivity from 3.3 to 11 and high uptake capacity for C 2 H 2 from 65.2 to 182 cm 3 g −1 (298K, 1 bar), an efficient separation is confirmed by breakthrough experiments. The near‐record high uptake for C 2 H 6 (166.8 cm 3 g −1 ) contributes to the promise for C 2 H 6 ‐selective separation of C 2 H 6 /C 2 H 4 . The multi‐module pore expansion enables transition from C 3 H 6 ‐selective to more desirable C 3 H 8 ‐selective separation with extraordinarily high C 3 H 8 uptake (254.9 cm 3 g −1 ) and high separation potential (1.25 mmol g −1 ) for C 3 H 8 /C 3 H 6 (50:50 v/v) mixture.
Related Topics
Concepts
Metal-organic framework
Materials science
Vanadium
Selectivity
Porosity
Gas separation
Mesoporous material
Sorption
Chemical engineering
Nanotechnology
Characterisation of pore space in soil
Metal
Crystallography
Physical chemistry
Organic chemistry
Adsorption
Chemistry
Composite material
Catalysis
Membrane
Engineering
Biochemistry
Metallurgy
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202403834
- OA Status
- green
- Cited By
- 36
- References
- 78
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4396749690
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4396749690Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adma.202403834Digital Object Identifier
- Title
-
Tailorable Multi‐Modular Pore‐Space‐Partitioned Vanadium Metal‐Organic Frameworks for Gas SeparationWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-05-08Full publication date if available
- Authors
-
Wei Wang, Yichong Chen, Pingyun Feng, Xianhui BuList of authors in order
- Landing page
-
https://doi.org/10.1002/adma.202403834Publisher landing page
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://www.osti.gov/biblio/2478388Direct OA link when available
- Concepts
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Metal-organic framework, Materials science, Vanadium, Selectivity, Porosity, Gas separation, Mesoporous material, Sorption, Chemical engineering, Nanotechnology, Characterisation of pore space in soil, Metal, Crystallography, Physical chemistry, Organic chemistry, Adsorption, Chemistry, Composite material, Catalysis, Membrane, Engineering, Biochemistry, MetallurgyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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36Total citation count in OpenAlex
- Citations by year (recent)
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2025: 24, 2024: 12Per-year citation counts (last 5 years)
- References (count)
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78Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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