Temperature-Driven Chemical Segregation in Co-Free Li-Rich-Layered Oxides and Its Influence on Electrochemical Performance Article Swipe
Kunkanadu R. Prakasha
,
Jêkabs Grîns
,
Aleksander Jaworski
,
Thomas Thersleff
,
Gunnar Svensson
,
Leif Olav Jøsang
,
Anne Dalager Dyrli
,
Andreas Paulus
,
Dries De Sloovere
,
Jan D’Haen
,
Marlies K. Van Bael
,
An Hardy
,
Hemesh Avireddy
,
J.R. Morante
,
Jordi Jacas Biendicho
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acs.chemmater.1c04150
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acs.chemmater.1c04150
Co-free Li-rich layered oxides are gaining interest as feasible positiveelectrode materials in lithium-ion batteries (LIBs) in terms of energy density, costreduction, and alleviating safety concerns. Unfortunately, their commercialization ishindered by severe structural degradation that occurs during electrochemical operation.The study at hand demonstrates advanced structural engineering of a Li-rich Co-freeoxide with composition Li1.1Ni0.35Mn0.55O2by spray pyrolysis and subsequentcalcination of an aqueous precursor, creating a segregated structure of two distinctlayered phases with space groupsR3??m(rhombohedral) andC2/m(monoclinic). Thisparticular structure was investigated with powder neutron diffraction, high-resolutionanalytical transmission electron microscopy imaging, and electron energy loss spectroscopic characterization. This complex structurecontributes to the high electrochemical stability and good rate capability observed for this compound (160 mAh/g at C/3 and 100mAh/g at 1C).These results provide new insights into the feasibility of developing and commercializing cobalt-free positiveelectrode materials for LIBs
Related Topics
Concepts
Materials science
Calcination
Monoclinic crystal system
Electrochemistry
Chemical engineering
Transmission electron microscopy
Lithium (medication)
Cobalt
Oxide
High-resolution transmission electron microscopy
Electrode
Crystal structure
Nanotechnology
Crystallography
Metallurgy
Catalysis
Physical chemistry
Chemistry
Medicine
Engineering
Endocrinology
Biochemistry
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.chemmater.1c04150
- OA Status
- green
- Cited By
- 13
- References
- 44
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4223547508
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4223547508Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.chemmater.1c04150Digital Object Identifier
- Title
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Temperature-Driven Chemical Segregation in Co-Free Li-Rich-Layered Oxides and Its Influence on Electrochemical PerformanceWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-04-11Full publication date if available
- Authors
-
Kunkanadu R. Prakasha, Jêkabs Grîns, Aleksander Jaworski, Thomas Thersleff, Gunnar Svensson, Leif Olav Jøsang, Anne Dalager Dyrli, Andreas Paulus, Dries De Sloovere, Jan D’Haen, Marlies K. Van Bael, An Hardy, Hemesh Avireddy, J.R. Morante, Jordi Jacas BiendichoList of authors in order
- Landing page
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https://doi.org/10.1021/acs.chemmater.1c04150Publisher landing page
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YesWhether a free full text is available
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-
greenOpen access status per OpenAlex
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https://hdl.handle.net/1942/37518Direct OA link when available
- Concepts
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Materials science, Calcination, Monoclinic crystal system, Electrochemistry, Chemical engineering, Transmission electron microscopy, Lithium (medication), Cobalt, Oxide, High-resolution transmission electron microscopy, Electrode, Crystal structure, Nanotechnology, Crystallography, Metallurgy, Catalysis, Physical chemistry, Chemistry, Medicine, Engineering, Endocrinology, BiochemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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13Total citation count in OpenAlex
- Citations by year (recent)
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2024: 5, 2023: 7, 2022: 1Per-year citation counts (last 5 years)
- References (count)
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44Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| corresponding_institution_ids | https://openalex.org/I4210128520 |
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