Temporal Separation between Lattice Dynamics and Electronic Spin‐State Switching in Spin‐Crossover Thin Films Evidenced by Time‐Resolved X‐Ray Diffraction Article Swipe
Karl Ridier
,
Roman Bertoni
,
Ritwika Mandal
,
Alix Volte
,
Yifeng Jiang
,
Elżbieta Trzop
,
Matteo Levantino
,
Yves Watier
,
Johannes Frey
,
Yuteng Zhang
,
Thomas Pézeril
,
H. Cailleau
,
Gábor Molnár
,
Azzedine Bousseksou
,
Maciej Lorenc
,
Céline Mariette
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202403585
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202403585
Spin‐crossover (SCO) complexes have drawn significant attention for the possibility to photoswitch their electronic spin state on a sub‐picosecond timescale at the molecular level. However, the multi‐step mechanism of laser‐pulse‐induced switching in solid state is not yet fully understood. Here, time‐resolved synchrotron X‐ray diffraction is used to follow the dynamics of the crystal lattice in response to a picosecond laser excitation in nanometric thin films of the SCO complex [Fe(HB(1,2,4‐triazol‐1‐yl) 3 ) 2 ]. The observed structural dynamics unambiguously reveal a lattice expansion on the 100 picosecond timescale, which is temporally decoupled both from the ultrafast molecular photoswitching process (occurring within 100 fs) and from the delayed, thermo‐elastic (Arrhenius‐driven) conversion (taking place ≈10 ns). These time‐separated dynamics are also manifested by the observation of damped acoustic oscillations in the time evolution of the lattice volume, whereas no such oscillations are observed in the electronic spin‐state dynamics. Overall, these results suggest the existence of a universal behavior whereby the intramolecular energy barrier between low‐spin and high‐spin states acts as an intrinsic dynamical bottleneck in the out‐of‐equilibrium spin‐state switching dynamics of SCO materials.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adfm.202403585
- OA Status
- hybrid
- Cited By
- 3
- References
- 50
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4400497682
All OpenAlex metadata
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https://openalex.org/W4400497682Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adfm.202403585Digital Object Identifier
- Title
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Temporal Separation between Lattice Dynamics and Electronic Spin‐State Switching in Spin‐Crossover Thin Films Evidenced by Time‐Resolved X‐Ray DiffractionWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-07-10Full publication date if available
- Authors
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Karl Ridier, Roman Bertoni, Ritwika Mandal, Alix Volte, Yifeng Jiang, Elżbieta Trzop, Matteo Levantino, Yves Watier, Johannes Frey, Yuteng Zhang, Thomas Pézeril, H. Cailleau, Gábor Molnár, Azzedine Bousseksou, Maciej Lorenc, Céline MarietteList of authors in order
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https://doi.org/10.1002/adfm.202403585Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1002/adfm.202403585Direct OA link when available
- Concepts
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Picosecond, Spin crossover, Materials science, Spin states, Femtosecond, Condensed matter physics, Diffraction, Excitation, Chemical physics, Laser, Physics, Optics, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
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3Total citation count in OpenAlex
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2025: 2, 2024: 1Per-year citation counts (last 5 years)
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50Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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