Terahertz-Driven Local Dipolar Correlation in a Quantum Paraelectric Article Swipe
Bing Cheng
,
Patrick L. Kramer
,
Zhi‐Xun Shen
,
Matthias C. Hoffmann
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1103/physrevlett.130.126902
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1103/physrevlett.130.126902
Light-induced ferroelectricity in quantum paraelectrics is a new avenue of achieving dynamic stabilization of hidden orders in quantum materials. In this Letter, we explore the possibility of driving a transient ferroelectric phase in the quantum paraelectric KTaO_{3} via intense terahertz excitation of the soft mode. We observe a long-lived relaxation in the terahertz-driven second harmonic generation (SHG) signal that lasts up to 20 ps at 10 K, which may be attributed to light-induced ferroelectricity. Through analyzing the terahertz-induced coherent soft-mode oscillation and finding its hardening with fluence well described by a single-well potential, we demonstrate that intense terahertz pulses up to 500 kV/cm cannot drive a global ferroelectric phase in KTaO_{3}. Instead, we find the unusual long-lived relaxation of the SHG signal comes from a terahertz-driven moderate dipolar correlation between the defect-induced local polar structures. We discuss the impact of our findings on current investigations of the terahertz-induced ferroelectric phase in quantum paraelectrics.
Related Topics
Concepts
Dipole
Terahertz radiation
Dielectric
Quantum correlation
Condensed matter physics
Quantum
Physics
Materials science
Quantum mechanics
Quantum discord
Quantum dynamics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1103/physrevlett.130.126902
- OA Status
- green
- Cited By
- 21
- References
- 29
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
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https://doi.org/10.1103/physrevlett.130.126902Digital Object Identifier
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Terahertz-Driven Local Dipolar Correlation in a Quantum ParaelectricWork title
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articleOpenAlex work type
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enPrimary language
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2023Year of publication
- Publication date
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2023-03-24Full publication date if available
- Authors
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Bing Cheng, Patrick L. Kramer, Zhi‐Xun Shen, Matthias C. HoffmannList of authors in order
- Landing page
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https://doi.org/10.1103/physrevlett.130.126902Publisher landing page
- Open access
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/1969708Direct OA link when available
- Concepts
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Dipole, Terahertz radiation, Dielectric, Quantum correlation, Condensed matter physics, Quantum, Physics, Materials science, Quantum mechanics, Quantum discord, Quantum dynamicsTop concepts (fields/topics) attached by OpenAlex
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21Total citation count in OpenAlex
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2025: 12, 2024: 5, 2023: 4Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| primary_location.is_oa | False |
| primary_location.source.id | https://openalex.org/S24807848 |
| primary_location.source.issn | 0031-9007, 1079-7114, 1092-0145 |
| primary_location.source.type | journal |
| primary_location.source.is_oa | False |
| primary_location.source.issn_l | 0031-9007 |
| primary_location.source.is_core | True |
| primary_location.source.is_in_doaj | False |
| primary_location.source.display_name | Physical Review Letters |
| primary_location.source.host_organization | https://openalex.org/P4310320261 |
| primary_location.source.host_organization_name | American Physical Society |
| primary_location.source.host_organization_lineage | https://openalex.org/P4310320261 |
| primary_location.source.host_organization_lineage_names | American Physical Society |
| primary_location.license | |
| primary_location.pdf_url | |
| primary_location.version | publishedVersion |
| primary_location.raw_type | journal-article |
| primary_location.license_id | |
| primary_location.is_accepted | True |
| primary_location.is_published | True |
| primary_location.raw_source_name | Physical Review Letters |
| primary_location.landing_page_url | https://doi.org/10.1103/physrevlett.130.126902 |
| publication_date | 2023-03-24 |
| publication_year | 2023 |
| referenced_works | https://openalex.org/W2138323937, https://openalex.org/W3120221077, https://openalex.org/W18219841, https://openalex.org/W2053483397, https://openalex.org/W2032018678, https://openalex.org/W2586965580, https://openalex.org/W4304144532, https://openalex.org/W2951821564, https://openalex.org/W2950022073, https://openalex.org/W3159284200, https://openalex.org/W1963893386, https://openalex.org/W2408812478, https://openalex.org/W2055076277, https://openalex.org/W2385034196, https://openalex.org/W2088506585, https://openalex.org/W2039146215, https://openalex.org/W2016062106, https://openalex.org/W2055612780, https://openalex.org/W2039997740, https://openalex.org/W2582750469, https://openalex.org/W1982860537, https://openalex.org/W2055654343, https://openalex.org/W2075941890, https://openalex.org/W1999952026, https://openalex.org/W2042384012, https://openalex.org/W2033093213, https://openalex.org/W2080149113, https://openalex.org/W1995401187, https://openalex.org/W2045391136 |
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| abstract_inverted_index.20 | 62 |
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| abstract_inverted_index.500 | 101 |
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| abstract_inverted_index.dipolar | 127 |
| abstract_inverted_index.discuss | 136 |
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| abstract_inverted_index.KTaO_{3} | 36 |
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| abstract_inverted_index.findings | 141 |
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| abstract_inverted_index.moderate | 126 |
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| abstract_inverted_index.ferroelectricity. | 73 |
| abstract_inverted_index.terahertz-induced | 77, 147 |
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| cited_by_percentile_year.min | 97 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 4 |
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| citation_normalized_percentile.is_in_top_10_percent | True |