Tetracycline removal from wastewater via g-C3N4 loaded RSM-CCD-optimised hybrid photocatalytic membrane reactor Article Swipe
YOU?
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· 2024
· Open Access
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· DOI: https://doi.org/10.1038/s41598-024-51847-5
In this study, a split-type photocatalytic membrane reactor (PMR), incorporating suspended graphitic carbon nitride (g-C3N4) as photocatalyst and a layered polymeric composite (using polyamide, polyethersulfone and polysulfone polymers) as a membrane was fabricated to remove tetracycline (TC) from aqueous solutions as the world's second most used and discharged antibiotic in wastewater. The photocatalyst was synthesised from melamine by ultrasonic-assisted thermal polymerisation method and, along with the membrane, was characterised using various methods, including Brunauer–Emmett–Teller analysis (BET), Fourier-transform infrared spectroscopy (FTIR), X-ray diffraction analysis (XRD), Field emission scanning electron microscopy (FESEM), and Ultraviolet–visible spectroscopy (UV–Vis). The PMR process was optimised, using Design-Expert software for tetracycline removal in terms of UV irradiation time, pH, photocatalyst loading, tetracycline concentration, and membrane separation iteration. It was revealed that a membrane-integrated reactor as a sustainable system could effectively produce clean water by simultaneous removal of tetracycline and photocatalyst from aqueous solution. The maximum removal of 94.8% was obtained at the tetracycline concentration of 22.16 ppm, pH of 9.78 with 0.56 g/L of photocatalyst in the irradiation time of 113.77 min after six times of passing membrane. The PMR system showed reasonable reusability by about a 25.8% drop in TC removal efficiency after seven cycles at optimal conditions. The outcomes demonstrate the promising performance of the proposed PMR system in tetracycline removal from water and suggest that it can be scaled as an effective approach for a sustainable supply of antibiotic-free clean water.
Related Topics
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41598-024-51847-5
- https://www.nature.com/articles/s41598-024-51847-5.pdf
- OA Status
- gold
- Cited By
- 37
- References
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- Related Works
- 10
- OpenAlex ID
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4390813804Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41598-024-51847-5Digital Object Identifier
- Title
-
Tetracycline removal from wastewater via g-C3N4 loaded RSM-CCD-optimised hybrid photocatalytic membrane reactorWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-01-12Full publication date if available
- Authors
-
Milad Esfandiaribayat, Mojtaba Binazadeh, Samad Sabbaghi, Milad Mohammadi, Samaneh Ghaedi, Hamid RajabiList of authors in order
- Landing page
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https://doi.org/10.1038/s41598-024-51847-5Publisher landing page
- PDF URL
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https://www.nature.com/articles/s41598-024-51847-5.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41598-024-51847-5.pdfDirect OA link when available
- Concepts
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Photocatalysis, Aqueous solution, Fourier transform infrared spectroscopy, Materials science, Tetracycline, Chemical engineering, Membrane, Nuclear chemistry, Melamine, Chemistry, Composite material, Organic chemistry, Catalysis, Antibiotics, Biochemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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37Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 25, 2024: 12Per-year citation counts (last 5 years)
- References (count)
-
77Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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