Tetraphenylethylene-embedded pillar[5]arene-based orthogonal self-assembly for efficient photocatalysis in water Article Swipe
Zhihang Bai
,
K. Velmurugan
,
Xueqi Tian
,
Minzan Zuo
,
Kaiya Wang
,
Xiao‐Yu Hu
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3762/bjoc.18.45
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3762/bjoc.18.45
Herein, we have designed and fabricated a simple and efficient supramolecular self-assembled nanosystem based on host–guest interactions between water-soluble tetraphenylethylene-embedded pillar[5]arene ( m -TPEWP5 ) and ammonium benzoyl-ʟ-alaninate ( G ) in an aqueous medium. The obtained assembly of m -TPEWP5 and G showed aggregation-induced emission (AIE) via the blocking of intramolecular phenyl-ring rotations and functioned as an ideal donor. After the loading of eosin Y ( EsY ) as acceptor on the surface of the assembly of m -TPEWP5 and G , the worm-like nanostructures changed into nanorods, which facilitates a Förster resonance energy transfer (FRET) from the m -TPEWP5 and G assembled donor to the EsY acceptor present in the nanorod assembly. The system comprising m -TPEWP5 , G and EsY displayed moderate FRET efficiency (31%) at a 2:1 molar ratio of donor-to-acceptor. Moreover, the obtained supramolecular nanorod assembly could act as a nanoreactor mimicking natural photosynthesis and exhibited a high catalytic efficiency for the photocatalytic dehalogenation reaction of various bromoketone derivatives with good yields in short reaction time in water.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3762/bjoc.18.45
- https://www.beilstein-journals.org/bjoc/content/pdf/1860-5397-18-45.pdf
- OA Status
- diamond
- Cited By
- 21
- References
- 37
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4224105956
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4224105956Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.3762/bjoc.18.45Digital Object Identifier
- Title
-
Tetraphenylethylene-embedded pillar[5]arene-based orthogonal self-assembly for efficient photocatalysis in waterWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-04-13Full publication date if available
- Authors
-
Zhihang Bai, K. Velmurugan, Xueqi Tian, Minzan Zuo, Kaiya Wang, Xiao‐Yu HuList of authors in order
- Landing page
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https://doi.org/10.3762/bjoc.18.45Publisher landing page
- PDF URL
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https://www.beilstein-journals.org/bjoc/content/pdf/1860-5397-18-45.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
diamondOpen access status per OpenAlex
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https://www.beilstein-journals.org/bjoc/content/pdf/1860-5397-18-45.pdfDirect OA link when available
- Concepts
-
Chemistry, Photocatalysis, Tetraphenylethylene, Pillar, Self-assembly, Nanotechnology, Combinatorial chemistry, Aggregation-induced emission, Organic chemistry, Catalysis, Materials science, Quantum mechanics, Physics, Structural engineering, Fluorescence, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
21Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 7, 2024: 5, 2023: 5, 2022: 4Per-year citation counts (last 5 years)
- References (count)
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37Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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