The Effect of sp2 Content in Carbon on Its Catalytic Activity for Acetylene Hydrochlorination Article Swipe
Fangjie Lu
,
Chengcheng Wei
,
Xue Yin
,
Lihua Kang
,
Mingyuan Zhu
,
Bin Dai
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/nano12152619
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/nano12152619
We report the influence of sp2 content in carbon catalyst on the catalytic activity for acetylene hydrochlorination. Nanodiamonds (NDs) were used as the precursor and calcinated under different temperatures. The resulting ND500, ND700, ND900, and ND1100 catalysts were characterized, and the sp2 content increased with increasing calcination temperature. The specific activities of the catalysts first increased and then decreased with increasing sp2 content. The highest catalytic activity could be obtained in the ND-900 catalyst with a sp2 value of 43.9%. The density functional theory results showed that the adsorption sites for acetylene and hydrogen chloride were located at the interface between sp2 and sp3 configuration.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/nano12152619
- https://www.mdpi.com/2079-4991/12/15/2619/pdf?version=1659346910
- OA Status
- gold
- Cited By
- 6
- References
- 26
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4289205465
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4289205465Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/nano12152619Digital Object Identifier
- Title
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The Effect of sp2 Content in Carbon on Its Catalytic Activity for Acetylene HydrochlorinationWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-07-29Full publication date if available
- Authors
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Fangjie Lu, Chengcheng Wei, Xue Yin, Lihua Kang, Mingyuan Zhu, Bin DaiList of authors in order
- Landing page
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https://doi.org/10.3390/nano12152619Publisher landing page
- PDF URL
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https://www.mdpi.com/2079-4991/12/15/2619/pdf?version=1659346910Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.mdpi.com/2079-4991/12/15/2619/pdf?version=1659346910Direct OA link when available
- Concepts
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Acetylene, Catalysis, Calcination, Adsorption, Carbon fibers, Hydrogen, Hydrogen chloride, Chemistry, Chemical engineering, Materials science, Inorganic chemistry, Organic chemistry, Composite number, Composite material, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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6Total citation count in OpenAlex
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2025: 3, 2023: 3Per-year citation counts (last 5 years)
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-
10Other works algorithmically related by OpenAlex
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