The Formation of Stacking Faults in Barium Zirconate-Type Perovskites Article Swipe
Dylan Jennings
,
Julian N. Ebert
,
Hongchu Du
,
Qianli Ma
,
Laura‐Alena Schäfer
,
Doris Sebold
,
Joachim Mayer
,
Wolfgang Rheinheimer
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/acs.chemmater.3c00787
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/acs.chemmater.3c00787
Yttrium-doped barium zirconate (BZY) is a proton-conducting perovskite with potential for use in a variety of energy applications, including as a catalyst support and as an electrolyte for solid-state fuel and electrolytic cells. Of interest to material performance is the presence and character of defects in the material, which will influence material properties. The presented work discusses the discovery of stacking faults in conventionally sintered BZY at different measured A/B ratios (BaxZr0.8Y0.2O3−δ, x = 0.989, 1.001, and 1.006). Two structurally unique stacking faults are observed for the first time in BZY, i.e., Ruddlesden–Popper (RP) type and non-RP type. Characterization using S/TEM details the presence of stacking faults and dislocations and provides insight into the formation process of RP-type faults in BZY-type materials. Electrochemical impedance spectroscopy is performed to analyze the impact of stacking faults on material conductivity. The stacking faults are concluded to be blocking conductivity and are expected to impact the mechanical properties of the material. The defects are also observed in a yttrium-doped barium zirconate/cerate (BZCY) with nickel oxide and are shown to be prevalent in close-to-stoichiometric BZY (A/B = 1.001), indicating that they are common defects for this material class.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.chemmater.3c00787
- OA Status
- hybrid
- Cited By
- 8
- References
- 80
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
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https://openalex.org/W4385568326Canonical identifier for this work in OpenAlex
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https://doi.org/10.1021/acs.chemmater.3c00787Digital Object Identifier
- Title
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The Formation of Stacking Faults in Barium Zirconate-Type PerovskitesWork title
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articleOpenAlex work type
- Language
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enPrimary language
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2023Year of publication
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2023-08-04Full publication date if available
- Authors
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Dylan Jennings, Julian N. Ebert, Hongchu Du, Qianli Ma, Laura‐Alena Schäfer, Doris Sebold, Joachim Mayer, Wolfgang RheinheimerList of authors in order
- Landing page
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https://doi.org/10.1021/acs.chemmater.3c00787Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1021/acs.chemmater.3c00787Direct OA link when available
- Concepts
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Yttrium, Materials science, Stacking, Perovskite (structure), Barium, Conductivity, Electrolyte, Oxide, Zirconate, Chemical engineering, Crystallography, Composite material, Ceramic, Metallurgy, Physical chemistry, Chemistry, Electrode, Engineering, Titanate, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
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8Total citation count in OpenAlex
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2025: 3, 2024: 4, 2023: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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