The Third Element Effect during Aqueous Corrosion of FeCrAl Alloys: Effect of Al Content Article Swipe
C.T. Lynch
,
Debashish Sur
,
Peter G. Connors
,
Benjamin W. Y. Redemann
,
Junsoo Han
,
Elizabeth J. Opila
,
John R. Scully
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1149/1945-7111/ae20c9
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1149/1945-7111/ae20c9
The third element effect draws on the synergy of some ternary systems. FeCrAl is one such alloy system that has shown superior high temperature oxidation resistance. However, the third element effect is understudied in aqueous corrosion. This study systematically explored the passivation behavior 4–16 at.% Al additions to single phase solid solution FeCr 10 alloys and compared their performance to Fe-Cr binary alloys. Additions of Al improved repassivation and long-term passivity of Fe (90-x) Cr 10 Al x alloys in deaerated acidified 0.1 M Na 2 SO 4 or 0.1 M H 2 SO 4 . Characterization via ex-situ X-ray photoelectron spectroscopy and in-operando atomic emission spectro-electrochemistry explored compositions of the films as well as the specific elemental dissolution kinetics into the electrolyte. Oxides or hydroxides consisting of Cr 2 O 3 , Cr(OH) 3 , and Al 2 O 3 improved passivation of Fe 90- x Cr 10 Al x alloys, relative to their ferrous and ferric oxides. The FeCr 10 Al 16 alloy composition behaved similarly to FeCr 16 when considering passivation performance. Even low concentrations of Al resulted in significant performance improvements in the passivity of FeCr 10 compared to binary Fe-Cr alloys with 16 at.% Cr. Discussion of the role of Al in the context of producing a third element effect, enhancing Cr (III) passivation, and as a secondary passivator itself is considered.
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- article
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- https://doi.org/10.1149/1945-7111/ae20c9
- OA Status
- hybrid
- References
- 48
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https://doi.org/10.1149/1945-7111/ae20c9Digital Object Identifier
- Title
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The Third Element Effect during Aqueous Corrosion of FeCrAl Alloys: Effect of Al ContentWork title
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articleOpenAlex work type
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2025Year of publication
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2025-11-18Full publication date if available
- Authors
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C.T. Lynch, Debashish Sur, Peter G. Connors, Benjamin W. Y. Redemann, Junsoo Han, Elizabeth J. Opila, John R. ScullyList of authors in order
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https://doi.org/10.1149/1945-7111/ae20c9Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1149/1945-7111/ae20c9Direct OA link when available
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0Total citation count in OpenAlex
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48Number of works referenced by this work
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| abstract_inverted_index.Fe-Cr | 60, 194 |
| abstract_inverted_index.X-ray | 99 |
| abstract_inverted_index.alloy | 16, 164 |
| abstract_inverted_index.draws | 4 |
| abstract_inverted_index.films | 111 |
| abstract_inverted_index.phase | 49 |
| abstract_inverted_index.shown | 20 |
| abstract_inverted_index.solid | 50 |
| abstract_inverted_index.study | 37 |
| abstract_inverted_index.their | 57, 154 |
| abstract_inverted_index.third | 1, 28, 212 |
| abstract_inverted_index.(90-x) | 73 |
| abstract_inverted_index.4–16 | 43 |
| abstract_inverted_index.Cr(OH) | 133 |
| abstract_inverted_index.FeCrAl | 12 |
| abstract_inverted_index.Oxides | 123 |
| abstract_inverted_index.alloys | 54, 78, 195 |
| abstract_inverted_index.atomic | 104 |
| abstract_inverted_index.binary | 61, 193 |
| abstract_inverted_index.effect | 3, 30 |
| abstract_inverted_index.ferric | 157 |
| abstract_inverted_index.itself | 224 |
| abstract_inverted_index.single | 48 |
| abstract_inverted_index.system | 17 |
| abstract_inverted_index.alloys, | 151 |
| abstract_inverted_index.alloys. | 62 |
| abstract_inverted_index.aqueous | 34 |
| abstract_inverted_index.behaved | 166 |
| abstract_inverted_index.context | 208 |
| abstract_inverted_index.effect, | 214 |
| abstract_inverted_index.element | 2, 29, 213 |
| abstract_inverted_index.ex-situ | 98 |
| abstract_inverted_index.ferrous | 155 |
| abstract_inverted_index.oxides. | 158 |
| abstract_inverted_index.synergy | 7 |
| abstract_inverted_index.ternary | 10 |
| abstract_inverted_index.However, | 26 |
| abstract_inverted_index.behavior | 42 |
| abstract_inverted_index.compared | 56, 191 |
| abstract_inverted_index.emission | 105 |
| abstract_inverted_index.explored | 39, 107 |
| abstract_inverted_index.improved | 66, 141 |
| abstract_inverted_index.kinetics | 119 |
| abstract_inverted_index.relative | 152 |
| abstract_inverted_index.resulted | 180 |
| abstract_inverted_index.solution | 51 |
| abstract_inverted_index.specific | 116 |
| abstract_inverted_index.superior | 21 |
| abstract_inverted_index.systems. | 11 |
| abstract_inverted_index.Additions | 63 |
| abstract_inverted_index.acidified | 81 |
| abstract_inverted_index.additions | 46 |
| abstract_inverted_index.deaerated | 80 |
| abstract_inverted_index.elemental | 117 |
| abstract_inverted_index.enhancing | 215 |
| abstract_inverted_index.long-term | 69 |
| abstract_inverted_index.oxidation | 24 |
| abstract_inverted_index.passivity | 70, 187 |
| abstract_inverted_index.producing | 210 |
| abstract_inverted_index.secondary | 222 |
| abstract_inverted_index.similarly | 167 |
| abstract_inverted_index.Discussion | 200 |
| abstract_inverted_index.consisting | 126 |
| abstract_inverted_index.corrosion. | 35 |
| abstract_inverted_index.hydroxides | 125 |
| abstract_inverted_index.passivator | 223 |
| abstract_inverted_index.composition | 165 |
| abstract_inverted_index.considered. | 226 |
| abstract_inverted_index.considering | 172 |
| abstract_inverted_index.dissolution | 118 |
| abstract_inverted_index.in-operando | 103 |
| abstract_inverted_index.passivation | 41, 142, 173 |
| abstract_inverted_index.performance | 58, 183 |
| abstract_inverted_index.resistance. | 25 |
| abstract_inverted_index.significant | 182 |
| abstract_inverted_index.temperature | 23 |
| abstract_inverted_index.compositions | 108 |
| abstract_inverted_index.electrolyte. | 122 |
| abstract_inverted_index.improvements | 184 |
| abstract_inverted_index.passivation, | 218 |
| abstract_inverted_index.performance. | 174 |
| abstract_inverted_index.spectroscopy | 101 |
| abstract_inverted_index.understudied | 32 |
| abstract_inverted_index.photoelectron | 100 |
| abstract_inverted_index.repassivation | 67 |
| abstract_inverted_index.concentrations | 177 |
| abstract_inverted_index.systematically | 38 |
| abstract_inverted_index.Characterization | 96 |
| abstract_inverted_index.spectro-electrochemistry | 106 |
| cited_by_percentile_year | |
| corresponding_author_ids | https://openalex.org/A5044464775, https://openalex.org/A5066250502, https://openalex.org/A5079079718, https://openalex.org/A5080982260, https://openalex.org/A5091385816, https://openalex.org/A5058175478, https://openalex.org/A5073061221 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 7 |
| corresponding_institution_ids | https://openalex.org/I145311948, https://openalex.org/I39804081, https://openalex.org/I4210092467, https://openalex.org/I4210104270, https://openalex.org/I51556381 |
| citation_normalized_percentile |