The local and average structure of Ba(Ti, Ce)O3 perovskite solid solution: effect of cerium concentration and particle size Article Swipe
Giorgia Confalonieri
,
Vincenzo Buscaglia
,
Giovanna Canu
,
María Teresa Buscaglia
,
Monica Dapiaggi
·
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.1107/s1600577519004508
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.1107/s1600577519004508
The amazing properties of ferroelectric perovskite BaTiO 3 (BT) and its solid solutions make them indispensable for many technological applications ( e.g. multilayer capacitors). Unfortunately, the so-called `size effect' limits their use. Indeed, under a certain critical particle size, these materials show a suppression of the spontaneous polarization and thus of the ferroelectric properties. In pure nanometric BaTiO 3 , this is related to a certain local structural disorder. However, only a few studies have explored BT solid solutions, where the doping effect, coupled to the reduced particle size, can play an important role. Therefore, in this work, the structure of BaCe x Ti 1– x O 3 ( x = 0.02–0.20) was explored by traditional Rietveld method and Pair Distribution Function. Samples present a particle size from 80–160 nm to 400–1000 nm depending on increasing x . The carbox approach was applied, investigating the evolution of the local structure, its modifications and the structural coherent correlation length, as a function of cerium amount. Results demonstrate a cooperative effect of composition and reduced size in the ferroelectricity loss. The two, in fact, contribute to intensify the local structural disorder, decreasing the structural coherent correlation length. The local structural disorder is thus confirmed to be a relevant factor in the ferroelectric properties degradation.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1107/s1600577519004508
- https://journals.iucr.org/s/issues/2019/04/00/co5124/co5124.pdf
- OA Status
- bronze
- Cited By
- 3
- References
- 33
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2952871227
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Raw OpenAlex JSON
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https://openalex.org/W2952871227Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1107/s1600577519004508Digital Object Identifier
- Title
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The local and average structure of Ba(Ti, Ce)O3 perovskite solid solution: effect of cerium concentration and particle sizeWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2019Year of publication
- Publication date
-
2019-06-06Full publication date if available
- Authors
-
Giorgia Confalonieri, Vincenzo Buscaglia, Giovanna Canu, María Teresa Buscaglia, Monica DapiaggiList of authors in order
- Landing page
-
https://doi.org/10.1107/s1600577519004508Publisher landing page
- PDF URL
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https://journals.iucr.org/s/issues/2019/04/00/co5124/co5124.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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bronzeOpen access status per OpenAlex
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https://journals.iucr.org/s/issues/2019/04/00/co5124/co5124.pdfDirect OA link when available
- Concepts
-
Ferroelectricity, Materials science, Particle size, Solid solution, Perovskite (structure), Rietveld refinement, Polarization (electrochemistry), Cerium, Chemical physics, Crystallography, Crystal structure, Chemistry, Physical chemistry, Dielectric, Optoelectronics, MetallurgyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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3Total citation count in OpenAlex
- Citations by year (recent)
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2023: 1, 2022: 1, 2020: 1Per-year citation counts (last 5 years)
- References (count)
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33Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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