The phenomenon of increasing capacitance induced by 1T/2H-MoS2 surface modification with Pt particles – Influence on composition and energy storage mechanism Article Swipe
Zuzanna Zarach
,
Mariusz Szkoda
,
Konrad Trzciński
,
Marcin Łapiński
,
Grzegorz Trykowski
,
Andrzej P. Nowak
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.electacta.2022.141389
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.electacta.2022.141389
In this paper, several approaches to the synthesis of molybdenum-based electrode materials for supercapacitors are presented, including anodization, hydrothermal process and annealing. For the material prepared via anodization of a molybdenum plate, followed by a hydrothermal process in thiourea aqueous solution, a thorough study of the Pt-surface modification through repetitive cycling in 1 M sulfuric acid with Pt acting as a counter electrode is performed, including X-ray photoelectron spectroscopy analysis and energy storage mechanism contribution. Along with the increasing number of cycles, an increase of the capacitance value is observed up to 1.064 F cm−2 after 60 000 cycles, resulting in more than tenfold growth (by over 1 150%). The analysis reveals progressive changes in the electrode material's chemical composition and the increasing pseudocapacitance contribution in energy storage processes, which is strictly caused by the formation of mixed molybdenum oxides with oxygen vacancies. Thus, Pt-surface modification effectively improves the electrochemical performance of the electrode material with excellent coulombic efficiency and capacitance retention. In a symmetric two-electrode configuration with Pt-modified electrode materials, the areal capacitance of 140.5 mF cm−2 is obtained after 50 000 cycles (with capacitance retention of 123%) indicating that Pt-surface modification of MoS2 may provide a novel approach for electrode materials for high-performance supercapacitors.
Related Topics
Concepts
Supercapacitor
Capacitance
Electrode
Pseudocapacitance
Materials science
Chemical engineering
Molybdenum
X-ray photoelectron spectroscopy
Electrochemistry
Faraday efficiency
Surface modification
Inorganic chemistry
Chemistry
Metallurgy
Engineering
Physical chemistry
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.electacta.2022.141389
- OA Status
- hybrid
- Cited By
- 30
- References
- 119
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4306880437
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4306880437Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.electacta.2022.141389Digital Object Identifier
- Title
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The phenomenon of increasing capacitance induced by 1T/2H-MoS2 surface modification with Pt particles – Influence on composition and energy storage mechanismWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-10-20Full publication date if available
- Authors
-
Zuzanna Zarach, Mariusz Szkoda, Konrad Trzciński, Marcin Łapiński, Grzegorz Trykowski, Andrzej P. NowakList of authors in order
- Landing page
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https://doi.org/10.1016/j.electacta.2022.141389Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
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https://doi.org/10.1016/j.electacta.2022.141389Direct OA link when available
- Concepts
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Supercapacitor, Capacitance, Electrode, Pseudocapacitance, Materials science, Chemical engineering, Molybdenum, X-ray photoelectron spectroscopy, Electrochemistry, Faraday efficiency, Surface modification, Inorganic chemistry, Chemistry, Metallurgy, Engineering, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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30Total citation count in OpenAlex
- Citations by year (recent)
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2025: 13, 2024: 10, 2023: 6, 2022: 1Per-year citation counts (last 5 years)
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119Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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