Theory of formability and diffusivity of point defects and impurites in Cd(Se,Te) Article Swipe
Anderson Janotti
,
Igor Evangelista
,
Intuon Chatratin
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.2172/2204850
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.2172/2204850
favor migration paths within the basal plane of the wurtzite CdS lattice, which may facilitate defect clustering and ultimately the formation of Cu-rich interfacial phases as observed by energy dispersive x-ray spectroscopic elemental maps in real PV devices. Se, Zn, and Sn defects are found to exhibit much larger activation energies and are not expected to diffuse within the CdS bulk at temperatures compatible with typical PV processing temperatures. Lastly, we find that Na interstitials are expected to exhibit slightly lower activation energies than K interstitials despite having a larger migration barrier. Still, we find both alkali species are expected to diffuse via an interstitially mediated mechanism at slightly higher temperatures than enable In, Ga, and Cu diffusion in the bulk. Our results indicate that processing temperatures in excess of ∼400 °C will lead to more interfacial intermixing with CdS buffer layers in CIGSe devices, and less so for CZTSSe absorbers where only Cu is expected to significantly diffuse into the buffer.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.2172/2204850
- OA Status
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- OpenAlex ID
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https://openalex.org/W4388534849Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.2172/2204850Digital Object Identifier
- Title
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Theory of formability and diffusivity of point defects and impurites in Cd(Se,Te)Work title
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articleOpenAlex work type
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enPrimary language
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2023Year of publication
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2023-10-26Full publication date if available
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Anderson Janotti, Igor Evangelista, Intuon ChatratinList of authors in order
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https://doi.org/10.2172/2204850Publisher landing page
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/2204850Direct OA link when available
- Concepts
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Materials science, Wurtzite crystal structure, Thermal diffusivity, Crystallographic defect, Activation energy, Diffusion, Lattice (music), Chemical physics, Condensed matter physics, Crystallography, Metallurgy, Thermodynamics, Chemistry, Physical chemistry, Zinc, Physics, AcousticsTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.typical | 65 |
| abstract_inverted_index.barrier. | 91 |
| abstract_inverted_index.devices, | 144 |
| abstract_inverted_index.devices. | 37 |
| abstract_inverted_index.energies | 50, 82 |
| abstract_inverted_index.expected | 54, 76, 99, 155 |
| abstract_inverted_index.indicate | 123 |
| abstract_inverted_index.lattice, | 11 |
| abstract_inverted_index.mediated | 105 |
| abstract_inverted_index.observed | 26 |
| abstract_inverted_index.slightly | 79, 108 |
| abstract_inverted_index.wurtzite | 9 |
| abstract_inverted_index.absorbers | 150 |
| abstract_inverted_index.diffusion | 117 |
| abstract_inverted_index.elemental | 32 |
| abstract_inverted_index.formation | 20 |
| abstract_inverted_index.mechanism | 106 |
| abstract_inverted_index.migration | 1, 90 |
| abstract_inverted_index.activation | 49, 81 |
| abstract_inverted_index.clustering | 16 |
| abstract_inverted_index.compatible | 63 |
| abstract_inverted_index.dispersive | 29 |
| abstract_inverted_index.facilitate | 14 |
| abstract_inverted_index.processing | 67, 125 |
| abstract_inverted_index.ultimately | 18 |
| abstract_inverted_index.interfacial | 23, 136 |
| abstract_inverted_index.intermixing | 137 |
| abstract_inverted_index.temperatures | 62, 110, 126 |
| abstract_inverted_index.interstitials | 74, 85 |
| abstract_inverted_index.significantly | 157 |
| abstract_inverted_index.spectroscopic | 31 |
| abstract_inverted_index.temperatures. | 68 |
| abstract_inverted_index.interstitially | 104 |
| cited_by_percentile_year | |
| countries_distinct_count | 1 |
| institutions_distinct_count | 3 |
| citation_normalized_percentile.value | 0.16532555 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |