Tip-enhanced Raman spectroscopy of confined carbon chains Article Swipe

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Cla Duri Tschannen , Thiago L. Vasconcelos , Lukáš Novotný ·

YOU? · · 2022 · Open Access · · DOI: https://doi.org/10.1063/5.0073950

Long linear chains of carbon encapsulated in carbon nanotubes represent the finite realization of carbyne, the truly one-dimensional carbon allotrope. Driven by advances in the synthesis of such structures, carbyne has attracted significant interest in recent years, with numerous experimental studies exploring its remarkable properties. As for other carbon nanomaterials, Raman spectroscopy has played an important role in the characterization of carbyne. In particular, tip-enhanced Raman scattering (TERS) has enabled imaging and spectroscopy down to the single-chain level. In this article, we provide a general introduction to carbyne and discuss the principles and experimental implementation of TERS as a key technology for the investigation of this material system. Within this context, the development of optical nanoantennas as TERS probes is addressed. We then summarize the latest progress in the Raman spectroscopic characterization of confined carbyne, with a focus on the findings assisted by TERS. Finally, we discuss open questions in the field and outline how TERS can contribute to solving them in future studies.

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Carbyne Raman spectroscopy Characterization (materials science) Context (archaeology) Materials science Nanotechnology Carbon nanotube Carbon fibers Raman scattering Carbon chain Spectroscopy Realization (probability) Chemistry Physics Optics Organic chemistry Composite number Composite material Paleontology Catalysis Mathematics Carbene Biology Statistics Quantum mechanics

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Type: article
Language: en
Landing Page: https://doi.org/10.1063/5.0073950
PDF: https://aip.scitation.org/doi/pdf/10.1063/5.0073950
OA Status: bronze
Cited By: 6
References: 84
Related Works: 10
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DOI: https://doi.org/10.1063/5.0073950

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Title: Tip-enhanced Raman spectroscopy of confined carbon chains

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Language: en

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Publication year: 2022

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Publication date: 2022-01-03

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Authors: Cla Duri Tschannen, Thiago L. Vasconcelos, Lukáš Novotný

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Landing page: https://doi.org/10.1063/5.0073950

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Concepts: Carbyne, Raman spectroscopy, Characterization (materials science), Context (archaeology), Materials science, Nanotechnology, Carbon nanotube, Carbon fibers, Raman scattering, Carbon chain, Spectroscopy, Realization (probability), Chemistry, Physics, Optics, Organic chemistry, Composite number, Composite material, Paleontology, Catalysis, Mathematics, Carbene, Biology, Statistics, Quantum mechanics

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Cited by: 6

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