To be or not to be a hydrophobic matrix? the role of coating hydrophobicity on anti-icing behavior and ions mobility of ionic liquids Article Swipe
Saba Goharshenas Moghadam
,
Gelareh Momen
,
Ehsan Bakhshandeh
,
Reza Jafari
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1016/j.cej.2024.149696
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1016/j.cej.2024.149696
The demand for anti-icing coatings to endure extremely low temperatures is substantial. Despite the innovative pioneering research on the anti-icing potential of ionic liquids (ILs), the development of such coatings is still in its infancy. Our study investigates how matrix hydrophobicity influences mobility of ILs at subzero temperatures and, consequently, their anti-icing behavior. Wettability results highlight the key role of IL anion hydrophobicity. Dielectric spectroscopy distinguishes ion mobility in the coatings at low temperatures. We also investigate how varying crosslink density affects ion mobility by measuring the water absorbency. Higher mobility of released ILs from the coatings at subzero was confirmed by their presence in water solutions, validated with UV–vis spectroscopy, and resulted in increased ionic conductivity. Differential scanning calorimetry and experimental setups were employed to assess ice formation temperature, time, and ice adhesion strength. Notably, surfaces containing IL exhibited a remarkable reduction in ice formation temperature to –23.5 ℃ and achieved an exceptionally low ice adhesion strength (∼15 kPa), attributed to the formation of a quasi-liquid layer (QLL). Solid-state NMR spectroscopy provided confirmation of the existence of QLL at the interface. Ice adhesion strength of coatings was examined against accelerated weathering, icing/de-icing cycles, as well as endurance against frost formation under freeze–thaw. Our findings underscore the significance of selecting the right matrix with regards to hydrophobicity and ILs when designing coatings for subfreezing applications.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.cej.2024.149696
- OA Status
- hybrid
- Cited By
- 18
- References
- 80
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4391940899
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4391940899Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.cej.2024.149696Digital Object Identifier
- Title
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To be or not to be a hydrophobic matrix? the role of coating hydrophobicity on anti-icing behavior and ions mobility of ionic liquidsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-02-20Full publication date if available
- Authors
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Saba Goharshenas Moghadam, Gelareh Momen, Ehsan Bakhshandeh, Reza JafariList of authors in order
- Landing page
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https://doi.org/10.1016/j.cej.2024.149696Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1016/j.cej.2024.149696Direct OA link when available
- Concepts
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Wetting, Ionic liquid, Differential scanning calorimetry, Chemical engineering, Materials science, Adhesion, Icing, Coating, Dielectric spectroscopy, Composite material, Chemistry, Organic chemistry, Electrochemistry, Physical chemistry, Meteorology, Thermodynamics, Catalysis, Physics, Engineering, ElectrodeTop concepts (fields/topics) attached by OpenAlex
- Cited by
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18Total citation count in OpenAlex
- Citations by year (recent)
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2025: 12, 2024: 6Per-year citation counts (last 5 years)
- References (count)
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80Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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