Toward Establishing Uniqueness of Experimentally Determined Transference Numbers Article Swipe
Darby T. Hickson
,
Nitash P. Balsara
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1149/1945-7111/adca04
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1149/1945-7111/adca04
The passage of current through a battery results in the development of concentration gradients in the electrolytic phase. For a fully characterized binary electrolyte, where the conductivity, salt diffusion coefficient, cation transference number, and the thermodynamic factor are known, concentration and potential gradients in the electrolytic phase can be modeled using Newman’s concentrated solution theory. We report two methods for measuring the transference number: the standard method based on electrochemical measurements ( ) and electrophoretic NMR ( ). The electrochemical approach requires combining measurements from multiple experiments; the equations used to determine the cation transference number and the thermodynamic factor are coupled, nonlinear algebraic equations. In the electrophoretic-NMR-based approach, however, the equations used to determine the cation transference number and the thermodynamic factor are decoupled. We find for a liquid electrolyte comprised of a lithium salt dissolved in tetraglyme, the values of the transference numbers obtained by these two methods are distinct. For example, at 30 °C, = −1.02 ± 1.11 and = 0.25 ± 0.04. The corresponding thermodynamic factors are also different. While the magnitude of the predicted concentration gradients based on the two sets of parameters are different, the predicted current-voltage relationships are similar.
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- Type
- article
- Language
- en
- Landing Page
- https://iopscience.iop.org/article/10.1149/1945-7111/adca04/pdf
- OA Status
- hybrid
- References
- 49
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4409231851
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Raw OpenAlex JSON
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https://openalex.org/W4409231851Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1149/1945-7111/adca04Digital Object Identifier
- Title
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Toward Establishing Uniqueness of Experimentally Determined Transference NumbersWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-04-01Full publication date if available
- Authors
-
Darby T. Hickson, Nitash P. BalsaraList of authors in order
- Landing page
-
https://iopscience.iop.org/article/10.1149/1945-7111/adca04/pdfPublisher landing page
- Open access
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://iopscience.iop.org/article/10.1149/1945-7111/adca04/pdfDirect OA link when available
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Uniqueness, Materials science, Mathematics, Mathematical analysisTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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49Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.electrophoretic | 92 |
| abstract_inverted_index.<mml:mi>t</mml:mi> | 77, 100, 198, 221 |
| abstract_inverted_index.<mml:mn>0</mml:mn> | 86, 109, 207, 230 |
| abstract_inverted_index.<mml:mo>+</mml:mo> | 80, 103, 201, 224 |
| abstract_inverted_index.<mml:mo>,</mml:mo> | 81, 104, 202, 225 |
| abstract_inverted_index.overflow="scroll"> | 74, 97, 195, 218 |
| abstract_inverted_index.electrophoretic-NMR-based | 143 |
| abstract_inverted_index.mathvariant="italic">eNMR</mml:mi> | 106, 227 |
| abstract_inverted_index.mathvariant="italic">echem</mml:mi> | 83, 204 |
| abstract_inverted_index.xmlns:mml="http://www.w3.org/1998/Math/MathML" | 73, 96, 194, 217 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 2 |
| citation_normalized_percentile.value | 0.09908257 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |