Transition path time over a barrier of a colloidal particle in a viscoelastic bath Article Swipe
Brandon R. Ferrer
,
Alejandro V. Arzola
,
Denis Boyer
,
Juan Ruben Gomez-Solano
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1103/physrevresearch.6.043237
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1103/physrevresearch.6.043237
We experimentally study the statistics of the transition path time taken by a submicron bead to successfully traverse an energy barrier created by two optical tweezers in two prototypical viscoelastic fluids, namely, aqueous polymer and micellar solutions. We find a very good agreement between our experimental distributions and a theoretical expression derived from the generalized Langevin equation for the particle motion. Our results reveal that the mean transition path times measured in such viscoelastic fluids have a nontrivial dependence on the barrier curvature and they can be significantly reduced when compared with those determined in Newtonian fluids of the same zero-shear viscosity. We verify that the decrease of the mean transition path time can be described in terms of an effective viscosity that quantitatively coincides with that measured by linear microrheology at a frequency determined by the reactive mode that gives rise to the unstable motion over the barrier. Therefore our results uncover the linear response of the particle during its thermally activated escape from a metastable state even when taking place in a non-Markovian bath. Published by the American Physical Society 2024
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1103/physrevresearch.6.043237
- OA Status
- gold
- Cited By
- 2
- References
- 108
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4404995405Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1103/physrevresearch.6.043237Digital Object Identifier
- Title
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Transition path time over a barrier of a colloidal particle in a viscoelastic bathWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-12-04Full publication date if available
- Authors
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Brandon R. Ferrer, Alejandro V. Arzola, Denis Boyer, Juan Ruben Gomez-SolanoList of authors in order
- Landing page
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https://doi.org/10.1103/physrevresearch.6.043237Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
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https://doi.org/10.1103/physrevresearch.6.043237Direct OA link when available
- Concepts
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Microrheology, Viscoelasticity, Viscosity, Particle (ecology), Curvature, Rheology, Metastability, Mechanics, Optical tweezers, Newtonian fluid, Physics, Materials science, Classical mechanics, Thermodynamics, Optics, Mathematics, Geology, Geometry, Quantum mechanics, OceanographyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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2Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2Per-year citation counts (last 5 years)
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108Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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