Tuning Higher Order Structure in Colloidal Fluids Article Swipe
Xiaoyue Wu
,
Fiona C. Meldrum
,
Katherine Skipper
,
Yushi Yang
,
C. Patrick Royall
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2303.09029
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2303.09029
Colloidal particles self assemble into a wide range of structures under external AC electric fields due to induced dipolar interactions [Yethiraj and Van Blaaderen Nature 421 513 (2003)]. As a result of these dipolar interactions, at low volume fraction the system is modulated between a hard-sphere like state (in the case of zero applied field) and a "string fluid" upon application of the field. Using both particle-resolved experiments and Brownian dynamics simulations, we investigate the emergence of the string fluid with a variety of structural measures including two-body and higher-order correlations. The higher-order structure we probe using three-body spatial correlation functions and a many-body approach based on minimum energy clusters of a dipolar-Lennard-Jones system. This yields a series of geometrically distinct minimum energy clusters upon increasing the strength of the dipolar interaction, which are echoed in the higher-order structure of the colloidal fluids we study here. We find good agreement between experiment and simulation at the two-body level, although some discrepancies are found at higher field strength, where the system falls out of equilibrium. Higher-order correlations exhibit reasonable agreement between experiment and simulation, again with more discrepancy at higher field strength for three--body correlation functions. At higher field strength, the cluster population in our experiments and simulations is dominated by the minimum energy clusters for all sizes $8 \leq m \leq 12$. The agreement that we find here is notable considering that there is no fit parameter in our mapping between experiment and simulation.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2303.09029
- https://arxiv.org/pdf/2303.09029
- OA Status
- green
- Cited By
- 1
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4327810449
All OpenAlex metadata
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https://openalex.org/W4327810449Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2303.09029Digital Object Identifier
- Title
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Tuning Higher Order Structure in Colloidal FluidsWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-03-16Full publication date if available
- Authors
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Xiaoyue Wu, Fiona C. Meldrum, Katherine Skipper, Yushi Yang, C. Patrick RoyallList of authors in order
- Landing page
-
https://arxiv.org/abs/2303.09029Publisher landing page
- PDF URL
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https://arxiv.org/pdf/2303.09029Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://arxiv.org/pdf/2303.09029Direct OA link when available
- Concepts
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Colloid, Chemical physics, Dipole, Cascade, Colloidal particle, Order (exchange), Short range order, Materials science, Range (aeronautics), Nanotechnology, Physics, Statistical physics, Condensed matter physics, Chemistry, Physical chemistry, Finance, Economics, Composite material, Quantum mechanics, ChromatographyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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1Total citation count in OpenAlex
- Citations by year (recent)
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2025: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.range | 7 |
| abstract_inverted_index.sizes | 216 |
| abstract_inverted_index.state | 47 |
| abstract_inverted_index.study | 144 |
| abstract_inverted_index.there | 232 |
| abstract_inverted_index.these | 32 |
| abstract_inverted_index.under | 10 |
| abstract_inverted_index.using | 96 |
| abstract_inverted_index.where | 167 |
| abstract_inverted_index.which | 132 |
| abstract_inverted_index.Nature | 24 |
| abstract_inverted_index.echoed | 134 |
| abstract_inverted_index.energy | 108, 122, 212 |
| abstract_inverted_index.field) | 54 |
| abstract_inverted_index.field. | 63 |
| abstract_inverted_index.fields | 14 |
| abstract_inverted_index.fluid" | 58 |
| abstract_inverted_index.fluids | 142 |
| abstract_inverted_index.higher | 164, 188, 196 |
| abstract_inverted_index.level, | 157 |
| abstract_inverted_index.result | 30 |
| abstract_inverted_index.series | 117 |
| abstract_inverted_index.string | 78 |
| abstract_inverted_index.system | 40, 169 |
| abstract_inverted_index.volume | 37 |
| abstract_inverted_index.yields | 115 |
| abstract_inverted_index."string | 57 |
| abstract_inverted_index.applied | 53 |
| abstract_inverted_index.between | 43, 150, 179, 240 |
| abstract_inverted_index.cluster | 200 |
| abstract_inverted_index.dipolar | 18, 33, 130 |
| abstract_inverted_index.exhibit | 176 |
| abstract_inverted_index.induced | 17 |
| abstract_inverted_index.mapping | 239 |
| abstract_inverted_index.minimum | 107, 121, 211 |
| abstract_inverted_index.notable | 229 |
| abstract_inverted_index.spatial | 98 |
| abstract_inverted_index.system. | 113 |
| abstract_inverted_index.variety | 82 |
| abstract_inverted_index.(2003)]. | 27 |
| abstract_inverted_index.Brownian | 69 |
| abstract_inverted_index.although | 158 |
| abstract_inverted_index.approach | 104 |
| abstract_inverted_index.assemble | 3 |
| abstract_inverted_index.clusters | 109, 123, 213 |
| abstract_inverted_index.distinct | 120 |
| abstract_inverted_index.dynamics | 70 |
| abstract_inverted_index.electric | 13 |
| abstract_inverted_index.external | 11 |
| abstract_inverted_index.fraction | 38 |
| abstract_inverted_index.measures | 85 |
| abstract_inverted_index.strength | 127, 190 |
| abstract_inverted_index.two-body | 87, 156 |
| abstract_inverted_index.Blaaderen | 23 |
| abstract_inverted_index.Colloidal | 0 |
| abstract_inverted_index.[Yethiraj | 20 |
| abstract_inverted_index.agreement | 149, 178, 223 |
| abstract_inverted_index.colloidal | 141 |
| abstract_inverted_index.dominated | 208 |
| abstract_inverted_index.emergence | 75 |
| abstract_inverted_index.functions | 100 |
| abstract_inverted_index.including | 86 |
| abstract_inverted_index.many-body | 103 |
| abstract_inverted_index.modulated | 42 |
| abstract_inverted_index.parameter | 236 |
| abstract_inverted_index.particles | 1 |
| abstract_inverted_index.strength, | 166, 198 |
| abstract_inverted_index.structure | 93, 138 |
| abstract_inverted_index.experiment | 151, 180, 241 |
| abstract_inverted_index.functions. | 194 |
| abstract_inverted_index.increasing | 125 |
| abstract_inverted_index.population | 201 |
| abstract_inverted_index.reasonable | 177 |
| abstract_inverted_index.simulation | 153 |
| abstract_inverted_index.structural | 84 |
| abstract_inverted_index.structures | 9 |
| abstract_inverted_index.three-body | 97 |
| abstract_inverted_index.application | 60 |
| abstract_inverted_index.considering | 230 |
| abstract_inverted_index.correlation | 99, 193 |
| abstract_inverted_index.discrepancy | 186 |
| abstract_inverted_index.experiments | 67, 204 |
| abstract_inverted_index.hard-sphere | 45 |
| abstract_inverted_index.investigate | 73 |
| abstract_inverted_index.simulation, | 182 |
| abstract_inverted_index.simulation. | 243 |
| abstract_inverted_index.simulations | 206 |
| abstract_inverted_index.three--body | 192 |
| abstract_inverted_index.Higher-order | 174 |
| abstract_inverted_index.correlations | 175 |
| abstract_inverted_index.equilibrium. | 173 |
| abstract_inverted_index.higher-order | 89, 92, 137 |
| abstract_inverted_index.interaction, | 131 |
| abstract_inverted_index.interactions | 19 |
| abstract_inverted_index.simulations, | 71 |
| abstract_inverted_index.correlations. | 90 |
| abstract_inverted_index.discrepancies | 160 |
| abstract_inverted_index.geometrically | 119 |
| abstract_inverted_index.interactions, | 34 |
| abstract_inverted_index.particle-resolved | 66 |
| abstract_inverted_index.dipolar-Lennard-Jones | 112 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 5 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
| sustainable_development_goals[0].score | 0.8199999928474426 |
| sustainable_development_goals[0].display_name | Affordable and clean energy |
| citation_normalized_percentile |