Tuning the Properties of MOF‐808 via Defect Engineering and Metal Nanoparticle Encapsulation Article Swipe
Rifan Hardian
,
Stefano Dissegna
,
Aladin Ullrich
,
Philip L. Llewellyn
,
Marie‐Vanessa Coulet
,
Roland A. Fischer
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1002/chem.202005050
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1002/chem.202005050
Defect engineering and metal encapsulation are considered as valuable approaches to fine‐tune the reactivity of metal–organic frameworks. In this work, various MOF‐808 (Zr) samples are synthesized and characterized with the final aim to understand how defects and/or platinum nanoparticle encapsulation act on the intrinsic and reactive properties of these MOFs. The reactivity of the pristine, defective and Pt encapsulated MOF‐808 is quantified with water adsorption and CO 2 adsorption calorimetry. The results reveal strong competitive effects between crystal morphology and missing linker defects which in turn affect the crystal morphology, porosity, stability, and reactivity. In spite of leading to a loss in porosity, the introduction of defects (missing linkers or Pt nanoparticles) is beneficial to the stability of the MOF‐808 towards water and could also be advantageously used to tune adsorption properties of this MOF family.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/chem.202005050
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/chem.202005050
- OA Status
- hybrid
- Cited By
- 86
- References
- 64
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3132064085
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3132064085Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/chem.202005050Digital Object Identifier
- Title
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Tuning the Properties of MOF‐808 via Defect Engineering and Metal Nanoparticle EncapsulationWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-02-14Full publication date if available
- Authors
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Rifan Hardian, Stefano Dissegna, Aladin Ullrich, Philip L. Llewellyn, Marie‐Vanessa Coulet, Roland A. FischerList of authors in order
- Landing page
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https://doi.org/10.1002/chem.202005050Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/chem.202005050Direct link to full text PDF
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/chem.202005050Direct OA link when available
- Concepts
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Encapsulation (networking), Nanoparticle, Materials science, Metal-organic framework, Nanotechnology, Chemical engineering, Chemistry, Computer science, Engineering, Organic chemistry, Computer network, AdsorptionTop concepts (fields/topics) attached by OpenAlex
- Cited by
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86Total citation count in OpenAlex
- Citations by year (recent)
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2025: 23, 2024: 19, 2023: 17, 2022: 23, 2021: 4Per-year citation counts (last 5 years)
- References (count)
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64Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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