Two-electron interference in two-photon attosecond double ionization of neon Article Swipe

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S. Chattopadhyay , Carlos Marante , Barry I. Schneider , C. William McCurdy , Luca Argenti ·

YOU? · · 2023 · Open Access · · DOI: https://doi.org/10.48550/arxiv.2312.09755

The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the transition between the non-sequential and sequential regime in two-photon double ionization (TPDI) is well explained by a virtual-sequential model. Much less is known, however, about the TPDI process in more complex atoms. Recently, we extended the virtual-sequential model to arbitrary light pulses [Chattopadhyay {\it et al.,} Phys. Rev. A~{\bf 108}, 013114 (2023)]. This extension employs multi-channel scattering states for the single ionization of both the neutral and the ionized target, which we initally applied to helium. In the present study, we show that our extended virtual-sequential model reproduces the qualitative features of the angularly integrated observables with available experimental results for neon, a considerably more complex target. We observe an intriguing feature of inverted two-particle interference in the joint energy distribution of $\mathrm{Ne}$ compared to $\mathrm{He}$. This phenomenon, attributable to the presence of a final doubly ionized state with triplet symmetry coupled to the two photoelectrons, should be observable with current experimental technologies.

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Attosecond Atomic physics Physics Ionization Neon Double ionization Observable Photoelectric effect Electron Helium Photon Laser Ion Optics Quantum mechanics Ultrashort pulse Argon

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Type: preprint
Language: en
Landing Page: http://arxiv.org/abs/2312.09755
PDF: https://arxiv.org/pdf/2312.09755
OA Status: green
Related Works: 10
OpenAlex ID: https://openalex.org/W4389912081

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DOI: https://doi.org/10.48550/arxiv.2312.09755

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Title: Two-electron interference in two-photon attosecond double ionization of neon

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Language: en

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Publication year: 2023

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Publication date: 2023-12-15

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Authors: S. Chattopadhyay, Carlos Marante, Barry I. Schneider, C. William McCurdy, Luca Argenti

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Landing page: https://arxiv.org/abs/2312.09755

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PDF URL: https://arxiv.org/pdf/2312.09755

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Concepts: Attosecond, Atomic physics, Physics, Ionization, Neon, Double ionization, Observable, Photoelectric effect, Electron, Helium, Photon, Laser, Ion, Optics, Quantum mechanics, Ultrashort pulse, Argon

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sustainable_development_goals[0].id	https://metadata.un.org/sdg/7
sustainable_development_goals[0].score	0.8999999761581421
sustainable_development_goals[0].display_name	Affordable and clean energy
citation_normalized_percentile